Nanoengineered Surfaces for Robust Droplet TENGs: Mitigating Contamination and Improving Longevity

IF 18.5 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Ying Ge, Huaifang Qin, Jingjing Wang, Jingjing Zhang, Zunkang Zhou, Yao Meng, Zanying Huang, Ke Yang, Zuliang Du, Peng Cui, Gang Cheng
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Abstract

The droplet triboelectric nanogenerator (D-TENG) harnesses energy from natural water droplets, though its performance and lifespan can be compromised by contamination on the functional layer. Water molecules have a strong affinity for polymer surfaces, which increases surface tension and the sliding-off angle, leading to greater droplet adhesion. As these droplets evaporate, they leave behind residues, such as calcium (Ca) and magnesium (Mg) salts, that obscure the polymer surface, thereby diminishing the electrification area and altering droplet dynamics—resulting in decreased electrical output. This study presents a micro-nanostructured D-TENG with advanced anti-fouling capabilities. By adding a layer of metal nanoparticles to the polymer surface, followed by ion etching and fluorination grafting, water retention and ion accumulation are effectively minimized. The anti-fouling D-TENG demonstrates a fourfold increase in electrical output compared to its predecessor. Following 10 000 droplet interactions, the output of the original D-TENG drops by 53%, whereas the anti-fouling variant only experiences a 7% reduction. These enhancements provide significant insights for D-TENG applications and contribute to the development of anti-fouling strategies.

Abstract Image

坚固液滴teng的纳米工程表面:减少污染和提高寿命
液滴摩擦电纳米发电机(D-TENG)利用天然水滴的能量,尽管其性能和寿命可能会受到功能层污染的影响。水分子对聚合物表面具有很强的亲和力,这增加了表面张力和滑动角,从而导致更大的液滴粘附。当这些液滴蒸发时,它们会留下诸如钙(Ca)和镁(Mg)盐之类的残留物,这些残留物会模糊聚合物表面,从而减少通电面积并改变液滴的动力学,从而导致电输出减少。本研究提出了一种具有先进防污能力的微纳米结构D-TENG。通过在聚合物表面添加一层金属纳米颗粒,然后进行离子蚀刻和氟化接枝,有效地减少了水潴留和离子积累。防污的D-TENG演示了四倍的电力输出相比,其前身。在10000个液滴相互作用后,原始D-TENG的产量下降了53%,而防污型只减少了7%。这些改进为D-TENG应用提供了重要的见解,并有助于防污策略的发展。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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