π-Conjugated Polymers for High-Performance Organic Electrochemical Transistors: Molecular Design Strategies, Applications and Perspectives

IF 16.1 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Dr. Zhicai Chen, Xinliang Ding, Junwei Wang, Prof. Xugang Guo, Prof. Shiyang Shao, Dr. Kui Feng
{"title":"π-Conjugated Polymers for High-Performance Organic Electrochemical Transistors: Molecular Design Strategies, Applications and Perspectives","authors":"Dr. Zhicai Chen,&nbsp;Xinliang Ding,&nbsp;Junwei Wang,&nbsp;Prof. Xugang Guo,&nbsp;Prof. Shiyang Shao,&nbsp;Dr. Kui Feng","doi":"10.1002/anie.202423013","DOIUrl":null,"url":null,"abstract":"<p>The last decade has witnessed significant progress in organic electrochemical transistors (OECTs) due to their enormous potential applications in various bioelectronic devices, such as artificial synapses, biological interfaces, and biosensors. The remarkable advance in this field is highly powered by the development of novel organic mixed ionic/electronic conductors (OMIECs). π-Conjugated polymers (CPs), which are widely used in various optoelectronics, are emerging as key channel materials for OECTs. In this review, after briefly introducing OECT, we then mainly focus on the latest progress in CPs for high-performance OECTs. The correlations of their structure, basic physicochemical properties, and device performance are elucidated by evaluating their electronic characters, optoelectronic properties, and OECT performance. Then, the applications of CP-based OECTs are briefly presented. Finally, we discuss several remaining issues or challenges in this field and give our insights into advancing CPs for enhanced OECT performance.</p>","PeriodicalId":125,"journal":{"name":"Angewandte Chemie International Edition","volume":"64 7","pages":""},"PeriodicalIF":16.1000,"publicationDate":"2025-01-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Angewandte Chemie International Edition","FirstCategoryId":"92","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/anie.202423013","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

The last decade has witnessed significant progress in organic electrochemical transistors (OECTs) due to their enormous potential applications in various bioelectronic devices, such as artificial synapses, biological interfaces, and biosensors. The remarkable advance in this field is highly powered by the development of novel organic mixed ionic/electronic conductors (OMIECs). π-Conjugated polymers (CPs), which are widely used in various optoelectronics, are emerging as key channel materials for OECTs. In this review, after briefly introducing OECT, we then mainly focus on the latest progress in CPs for high-performance OECTs. The correlations of their structure, basic physicochemical properties, and device performance are elucidated by evaluating their electronic characters, optoelectronic properties, and OECT performance. Then, the applications of CP-based OECTs are briefly presented. Finally, we discuss several remaining issues or challenges in this field and give our insights into advancing CPs for enhanced OECT performance.

Abstract Image

高性能有机电化学晶体管用π共轭聚合物:分子设计策略、应用与展望
由于有机电化学晶体管(OECTs)在人工突触、生物界面和生物传感器等各种生物电子器件中具有巨大的应用潜力,在过去的十年中取得了重大进展。新型有机混合离子/电子导体(OMIECs)的发展极大地推动了这一领域取得的显著进展。其中,π共轭聚合物(CPs)广泛应用于各种光电子领域,正成为oect的关键通道材料。本文在简要介绍OECT的基础上,重点介绍了高性能OECT的CPs的最新进展。通过评价它们的电子特性、光电特性和OECT性能,进一步阐明了它们的结构、基本物理化学性质和器件性能之间的相关性。然后简要介绍了基于cp的oect的应用。最后,我们讨论了该领域的几个遗留问题或挑战,并给出了我们对推进cp以提高OECT性能的见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
CiteScore
26.60
自引率
6.60%
发文量
3549
审稿时长
1.5 months
期刊介绍: Angewandte Chemie, a journal of the German Chemical Society (GDCh), maintains a leading position among scholarly journals in general chemistry with an impressive Impact Factor of 16.6 (2022 Journal Citation Reports, Clarivate, 2023). Published weekly in a reader-friendly format, it features new articles almost every day. Established in 1887, Angewandte Chemie is a prominent chemistry journal, offering a dynamic blend of Review-type articles, Highlights, Communications, and Research Articles on a weekly basis, making it unique in the field.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信