Unlocking Zero Liquid Discharge: A Parallel Water Supply Strategy to Realize Selective Salt Crystallization for Long-Term Interfacial Solar Evaporation

IF 18.5 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Qianqian Xiong, Deyu Wang, Bo Shao, Huimin Yu, Xuan Wu, Yi Lu, Xiaofei Yang, Haolan Xu
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Abstract

Interfacial solar evaporation offers a green and sustainable solution to solve clean water shortages via solar-driven desalination. However, salt crystallization and accumulation on solar evaporators have become the primary hindrances to the long-term practical application of interfacial solar evaporation technology. To tackle this challenge, a photothermal evaporator with a novel parallel two-water paths strategy is developed in this study. Unlike the conventional one-way water path, which generally leads to salt accumulation at the water supply end on the evaporation surfaces, thereby limiting the lifespan of the evaporator and compromising solar evaporation performance, here, with the second parallel water supply path, the ion diffusion and distribution within the solar evaporator is reconfigured and optimized. No salt accumulation occurs on either the evaporation surfaces or the water paths, eliminating the impact of salt crystallization on evaporation performance and enabling convenient salt collection. A high and stable evaporation rate of 3.09–3.26 kg m−2 h−1 is recorded over 84 h continuous evaporation of NaCl solution (3.5 wt.%) without salt accumulation on the evaporator, making it an ideal strategy for zero liquid discharge solar evaporation.

Abstract Image

Abstract Image

解锁零液体排放:实现长期界面太阳蒸发选择性盐结晶的平行供水策略
界面太阳能蒸发提供了一种绿色和可持续的解决方案,通过太阳能驱动的海水淡化来解决清洁水短缺问题。然而,太阳能蒸发器上盐的结晶和积累已成为界面太阳能蒸发技术长期实际应用的主要障碍。为了解决这一挑战,本研究开发了一种具有新型平行双水路策略的光热蒸发器。传统的单向水路径通常会导致供水端在蒸发表面积聚盐分,从而限制蒸发器的使用寿命并影响太阳能蒸发性能,与此不同的是,在第二平行供水路径中,太阳能蒸发器内部的离子扩散和分布被重新配置和优化。蒸发表面和水路均不发生盐积累,消除了盐结晶对蒸发性能的影响,方便了盐的收集。NaCl溶液(3.5 wt.%)连续蒸发84 h,蒸发器上无盐积累,蒸发速率为3.09 ~ 3.26 kg m−2 h−1,是理想的零液体排放太阳能蒸发策略。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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