{"title":"An Urchin-Inspired Broadband and Ultralight Microwave Absorber","authors":"You Zhang, Xiaofeng Gong, Yanan Zeng, Xingjun Dong, Hui Guo, Zhenhua Jiang, Tianjiao Hu, Jing Wang, Yanhong Zou, Zengyong Chu","doi":"10.1002/adfm.202419943","DOIUrl":null,"url":null,"abstract":"<p>The incompatibility between low and high frequencies, and the constraints of thickness and absorption bandwidth, are great challenges for electromagnetic wave (EMW) absorbers. The combination of microscopic wrinkled morphology and macroscopic stacking structure offers the possibility of constructing lightweight and broadband EMW-absorbing materials. Herein an artificial periodic unit is demonstrated, wCNT@PS/R, which consists of the urchin-inspired wrinkled-carbon nanotube (CNT)-coated polystyrene (PS) spheres and the organosilicon rubber matrix. The unit thickness and the unit geometry are studied and optimized. Due to the good impedance matching, excellent macrostructural reflections, and strong dielectric loss, the pentagon unit achieves a promising effect absorption band (EAB) of 12.61 GHz, covering both the low-frequency (S- and C-band) and the high-frequency (X- and Ku-band) bands. The thickness is 4.0 mm and the total density is as low as 0.194 g cm<sup>−3</sup>, which provides a new idea for the cost-effective preparation of thin, ultralight, and broadband EMW absorbers.</p>","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"35 19","pages":""},"PeriodicalIF":19.0000,"publicationDate":"2025-01-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Functional Materials","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/adfm.202419943","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The incompatibility between low and high frequencies, and the constraints of thickness and absorption bandwidth, are great challenges for electromagnetic wave (EMW) absorbers. The combination of microscopic wrinkled morphology and macroscopic stacking structure offers the possibility of constructing lightweight and broadband EMW-absorbing materials. Herein an artificial periodic unit is demonstrated, wCNT@PS/R, which consists of the urchin-inspired wrinkled-carbon nanotube (CNT)-coated polystyrene (PS) spheres and the organosilicon rubber matrix. The unit thickness and the unit geometry are studied and optimized. Due to the good impedance matching, excellent macrostructural reflections, and strong dielectric loss, the pentagon unit achieves a promising effect absorption band (EAB) of 12.61 GHz, covering both the low-frequency (S- and C-band) and the high-frequency (X- and Ku-band) bands. The thickness is 4.0 mm and the total density is as low as 0.194 g cm−3, which provides a new idea for the cost-effective preparation of thin, ultralight, and broadband EMW absorbers.
低频与高频的不兼容,以及厚度和吸收带宽的限制,是电磁波吸收器面临的巨大挑战。微观皱褶形态与宏观堆积结构的结合,为构建轻量化宽频带电磁吸波材料提供了可能。本文演示了一个人工周期单元wCNT@PS/R,它由海胆启发的褶皱碳纳米管(CNT)包覆聚苯乙烯(PS)球和有机硅橡胶基体组成。对单元厚度和单元几何进行了研究和优化。由于五角形单元具有良好的阻抗匹配、优异的宏观反射和较强的介电损耗,使得五角形单元在12.61 GHz的效果吸收波段(EAB)具有广阔的应用前景,覆盖低频(S波段和c波段)和高频(X波段和ku波段)。厚度为4.0 mm,总密度低至0.194 g cm−3,为制备超薄、超轻、宽带EMW吸波材料提供了新的思路。
期刊介绍:
Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week.
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