Highly Sensitive Low-Frequency Acoustic Sensor Based on Functionalized Graphene Oxide

IF 13 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Small Pub Date : 2024-12-31 DOI:10.1002/smll.202409043
Anqi Chen, Lin Xi, Tianyu Li, Xiaona Du, Xiaoyan Zhang, Lili Hou
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Abstract

Developing miniaturized low-frequency acoustic sensors with high sensitivity is crucial for diverse applications, including geological monitoring and aerospace exploration. However, the performance of low-frequency acoustic sensor is constrained by the limited mechanical robustness of traditional sensing films at nanoscale thickness. Here, a functionalized graphene oxide (GO)-based Fabry-Perot (FP) low-frequency sensor is proposed, with characteristics of compact size, resistance to electromagnetic interference high-sensitivity low minimum detectable pressure (MDP), and a high signal-to-noise ratio (SNR). The functionalized GO is synthesized through the reaction of GO with dodecylamine and the uniform film is prepared by a self-assembly method. This sensor exhibits a sensitivity of −91.92 dB re 1 rad/µPa at 10–200 Hz with a fluctuation of 0.4 dB, ≈5.6 times higher than that of non-functionalized GO-based sensors prepared by a direct evaporation method. The MDP of this sensor is determined to be 0.333 µPa/Hz1/2 @20 Hz with a SNR of 136.34 dB, which outperforms previously reported low-frequency sensors using conventional metals or polymers as sensing films.

Abstract Image

基于功能化氧化石墨烯的高灵敏度低频声传感器
开发具有高灵敏度的小型化低频声传感器对于多种应用至关重要,包括地质监测和航空航天勘探。然而,传统传感膜在纳米尺度下的机械鲁棒性有限,限制了低频声传感器的性能。本文提出了一种基于功能化氧化石墨烯(GO)的Fabry-Perot (FP)低频传感器,该传感器具有体积小、抗电磁干扰、高灵敏度、低可探测压力(MDP)和高信噪比(SNR)的特点。通过氧化石墨烯与十二烷基胺反应合成功能化氧化石墨烯,并采用自组装法制备均匀膜。该传感器在10-200 Hz下的灵敏度为- 91.92 dB re 1 rad/µPa,波动为0.4 dB,比直接蒸发法制备的非功能化氧化石墨烯传感器高约5.6倍。该传感器的MDP为0.333 μ Pa/Hz1/2 @20 Hz,信噪比为136.34 dB,优于先前报道的使用传统金属或聚合物作为传感膜的低频传感器。
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来源期刊
Small
Small 工程技术-材料科学:综合
CiteScore
17.70
自引率
3.80%
发文量
1830
审稿时长
2.1 months
期刊介绍: Small serves as an exceptional platform for both experimental and theoretical studies in fundamental and applied interdisciplinary research at the nano- and microscale. The journal offers a compelling mix of peer-reviewed Research Articles, Reviews, Perspectives, and Comments. With a remarkable 2022 Journal Impact Factor of 13.3 (Journal Citation Reports from Clarivate Analytics, 2023), Small remains among the top multidisciplinary journals, covering a wide range of topics at the interface of materials science, chemistry, physics, engineering, medicine, and biology. Small's readership includes biochemists, biologists, biomedical scientists, chemists, engineers, information technologists, materials scientists, physicists, and theoreticians alike.
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