{"title":"Strain Effects in Carbon Dioxide Electroreduction","authors":"Siying Zhang, Weidong Ruan, Jingqi Guan","doi":"10.1002/aenm.202404057","DOIUrl":null,"url":null,"abstract":"<p>As a frontier method for adjusting the electronic and geometric configurations of metal sites, lattice strain engineering plays a key role in regulating the interaction between catalytic surface and adsorbed molecules. Here, the research progress of strain effects in electrochemical carbon dioxide reduction (CO<sub>2</sub>RR) is reviewed. Starting from the basic principles of strain effects in the CO<sub>2</sub>RR, the advanced in situ characterization techniques are summarized. The key effect of strain on the structure–activity relationship in CO<sub>2</sub>RR is comprehensively discussed. Subsequently, the electrocatalysts with different properties rich in strain are classified, including core–shell structure catalysts, alloys, transition metal compounds, and single-atom catalysts. Finally, the obstacles encountered in the practical application of strain effect are proposed, and the future research direction of this emerging field is prospected.</p>","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"15 14","pages":""},"PeriodicalIF":26.0000,"publicationDate":"2024-12-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Energy Materials","FirstCategoryId":"88","ListUrlMain":"https://advanced.onlinelibrary.wiley.com/doi/10.1002/aenm.202404057","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
As a frontier method for adjusting the electronic and geometric configurations of metal sites, lattice strain engineering plays a key role in regulating the interaction between catalytic surface and adsorbed molecules. Here, the research progress of strain effects in electrochemical carbon dioxide reduction (CO2RR) is reviewed. Starting from the basic principles of strain effects in the CO2RR, the advanced in situ characterization techniques are summarized. The key effect of strain on the structure–activity relationship in CO2RR is comprehensively discussed. Subsequently, the electrocatalysts with different properties rich in strain are classified, including core–shell structure catalysts, alloys, transition metal compounds, and single-atom catalysts. Finally, the obstacles encountered in the practical application of strain effect are proposed, and the future research direction of this emerging field is prospected.
期刊介绍：
Established in 2011, Advanced Energy Materials is an international, interdisciplinary, English-language journal that focuses on materials used in energy harvesting, conversion, and storage. It is regarded as a top-quality journal alongside Advanced Materials, Advanced Functional Materials, and Small.
With a 2022 Impact Factor of 27.8, Advanced Energy Materials is considered a prime source for the best energy-related research. The journal covers a wide range of topics in energy-related research, including organic and inorganic photovoltaics, batteries and supercapacitors, fuel cells, hydrogen generation and storage, thermoelectrics, water splitting and photocatalysis, solar fuels and thermosolar power, magnetocalorics, and piezoelectronics.
The readership of Advanced Energy Materials includes materials scientists, chemists, physicists, and engineers in both academia and industry. The journal is indexed in various databases and collections, such as Advanced Technologies & Aerospace Database, FIZ Karlsruhe, INSPEC (IET), Science Citation Index Expanded, Technology Collection, and Web of Science, among others.
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