Yang You, Hanye Xing, Kangkang Li, Yuqing Xie, Meiqi Ye, Yang Lu, Jingzhe Xue
{"title":"Bioinspired Carbon‐Silver Sulfide Scaffold with Synergistic Enhanced Light Capture and Anti‐Biofouling Property for Stable Solar Steam Generation","authors":"Yang You, Hanye Xing, Kangkang Li, Yuqing Xie, Meiqi Ye, Yang Lu, Jingzhe Xue","doi":"10.1002/smll.202402544","DOIUrl":null,"url":null,"abstract":"Carbon material is a hot topic in solar evaporation. Due to the widely distributed microorganisms in natural water, biofouling has limited the actual application of solar evaporation material. Although carbon material lacks of nutrition for microbe, it is still vulnerable to biofouling because of the efficient pollutant adsorption property. However, current anti‐biofouling design focuses on microbial control, neglects its influence on evaporators light absorption, that is usually a trade‐off with evaporation efficiency. Herein, a bioinspired aligned carbon‐Ag<jats:sub>2</jats:sub>S scaffold is introduced with synergistical enhanced light absorption (increased to 98.0% from 97.4%) and anti‐biofouling property. The bioinspired aligned carbon‐Ag<jats:sub>2</jats:sub>S scaffold exhibits a 1.87 kg m<jats:sup>−2</jats:sup> h<jats:sup>−1</jats:sup> evaporation rate under one sun, superior to pure carbon scaffold (1.78 kg m<jats:sup>−2</jats:sup> h<jats:sup>−1</jats:sup>). It also maintains efficient light capture (‐97.2%) and evaporation rate (1.73 kg m<jats:sup>−2</jats:sup> h<jats:sup>−1</jats:sup>) after bacterial interference, avoiding sharp decline in light absorption (reduced to 83.3–87.6%) and evaporation performance (reduced to 1.24–1.28 kg m<jats:sup>−2</jats:sup> h<jats:sup>−1</jats:sup>) which occurs in carbon scaffold due to biofouling. The carbon‐Ag<jats:sub>2</jats:sub>S scaffold shows solid advantage in balancing light captures and biofouling control, compared to carbon‐ZnO scaffold with conventional anti‐biofouling design, which inhibits biofouling sacrificing light absorption (reduced to 89.8%) and evaporation performance (reduced to 1.41 kg m<jats:sup>−2</jats:sup> h<jats:sup>−1</jats:sup>).","PeriodicalId":228,"journal":{"name":"Small","volume":"244 6 1","pages":""},"PeriodicalIF":13.0000,"publicationDate":"2024-12-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Small","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/smll.202402544","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Carbon material is a hot topic in solar evaporation. Due to the widely distributed microorganisms in natural water, biofouling has limited the actual application of solar evaporation material. Although carbon material lacks of nutrition for microbe, it is still vulnerable to biofouling because of the efficient pollutant adsorption property. However, current anti‐biofouling design focuses on microbial control, neglects its influence on evaporators light absorption, that is usually a trade‐off with evaporation efficiency. Herein, a bioinspired aligned carbon‐Ag2S scaffold is introduced with synergistical enhanced light absorption (increased to 98.0% from 97.4%) and anti‐biofouling property. The bioinspired aligned carbon‐Ag2S scaffold exhibits a 1.87 kg m−2 h−1 evaporation rate under one sun, superior to pure carbon scaffold (1.78 kg m−2 h−1). It also maintains efficient light capture (‐97.2%) and evaporation rate (1.73 kg m−2 h−1) after bacterial interference, avoiding sharp decline in light absorption (reduced to 83.3–87.6%) and evaporation performance (reduced to 1.24–1.28 kg m−2 h−1) which occurs in carbon scaffold due to biofouling. The carbon‐Ag2S scaffold shows solid advantage in balancing light captures and biofouling control, compared to carbon‐ZnO scaffold with conventional anti‐biofouling design, which inhibits biofouling sacrificing light absorption (reduced to 89.8%) and evaporation performance (reduced to 1.41 kg m−2 h−1).
期刊介绍:
Small serves as an exceptional platform for both experimental and theoretical studies in fundamental and applied interdisciplinary research at the nano- and microscale. The journal offers a compelling mix of peer-reviewed Research Articles, Reviews, Perspectives, and Comments.
With a remarkable 2022 Journal Impact Factor of 13.3 (Journal Citation Reports from Clarivate Analytics, 2023), Small remains among the top multidisciplinary journals, covering a wide range of topics at the interface of materials science, chemistry, physics, engineering, medicine, and biology.
Small's readership includes biochemists, biologists, biomedical scientists, chemists, engineers, information technologists, materials scientists, physicists, and theoreticians alike.