Enhancing Hole Extraction and Transfer via Phthalocyanine-Assisted Hole Transport Material for High-Performance Perovskite Solar Cells

IF 7.1 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY

ACS Sustainable Chemistry & Engineering Pub Date : 2024-12-12 DOI:10.1021/acssuschemeng.4c0752410.1021/acssuschemeng.4c07524

Min Xu, Liangding Zheng, Peng Wang, Shihuai Wang*, Lin Xie* and Yong Hua*,

引用次数: 0

Abstract

Enhancing hole extraction and transfer of the hole transport layer (HTL) is urgently needed to achieve excellent performance perovskite solar cells. Herein, a novel phthalocyanine (TQ) has been introduced into Spiro-OMeTAD to finely optimize the hole transport properties of the HTL for achieving better performance. It is demonstrated that TQ incorporation can effectively enhance hole extraction/transfer and reduce charge recombination in the device. The TQ-treated device yields an improved power conversion efficiency of 24.29% from 21.91%. Remarkably, these unencapsulated devices demonstrate remarkable moisture, light, and thermal stabilities.

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来源期刊

ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL

CiteScore

13.80

自引率

4.80%

发文量

1470

审稿时长

1.7 months

期刊介绍： ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.