CO2 Capture Using Resin-Based Solid Amines: Characteristic, Application, Regeneration and Deactivation Mechanism

IF 8.1 1区 工程技术 Q1 ENGINEERING, CHEMICAL
Endian Hu, Li Lin, Kailun Chen, Jinglin Li, Yuchen Gao, Jingwen Chang, Weikai Qin, Yukun Zhao, Jianguo Jiang
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Abstract

The accumulation of CO2 has been considered to be one of the main contributors to global warming and climate change, making carbon emission reduction and carbon capture technologies key research focuses. Out of the various technologies to lower atmospheric CO2 levels, using solid amine adsorbents for CO2 capture is seen as one of the most promising options. Porous resin materials are gradually being investigated as porous solid supports for amine functionalization due to their high specific surface area and high adsorption properties. In this review, we focus on the application of resin-based solid amines in carbon capture, offer a detailed overview of the synthesis methods for resin-based solid amines, and discuss how different supports and organic amines impact the performance of these adsorbent materials. We explore factors affecting the stability of these materials, including deactivation caused by heat, moisture, oxidation, CO2, and impurity gases, to identify the causes and mechanisms of deactivation, and providing the thorough summary of how resin-based solid amines perform in CO2 adsorption under various environmental conditions. Our review addresses a gap of resin supports in the current literature on solid amine adsorbents.

Abstract Image

Abstract Image

树脂基固体胺捕集CO2:特性、应用、再生及失活机理
二氧化碳的积累被认为是导致全球变暖和气候变化的主要因素之一,因此碳减排和碳捕集技术成为研究的重点。在各种降低大气二氧化碳水平的技术中,使用固体胺吸附剂捕获二氧化碳被认为是最有前途的选择之一。多孔树脂材料因其高比表面积和高吸附性能而逐渐成为胺类功能化的多孔固体载体。本文重点介绍了树脂基固体胺在碳捕获中的应用,详细介绍了树脂基固体胺的合成方法,并讨论了不同载体和有机胺对这些吸附材料性能的影响。我们探讨了影响这些材料稳定性的因素,包括热、湿、氧化、CO2和杂质气体引起的失活,以确定失活的原因和机制,并对树脂基固体胺在各种环境条件下如何吸附CO2进行了全面的总结。我们的审查解决了树脂支持在固体胺吸附剂目前的文献差距。
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来源期刊
Separation and Purification Technology
Separation and Purification Technology 工程技术-工程:化工
CiteScore
14.00
自引率
12.80%
发文量
2347
审稿时长
43 days
期刊介绍: Separation and Purification Technology is a premier journal committed to sharing innovative methods for separation and purification in chemical and environmental engineering, encompassing both homogeneous solutions and heterogeneous mixtures. Our scope includes the separation and/or purification of liquids, vapors, and gases, as well as carbon capture and separation techniques. However, it's important to note that methods solely intended for analytical purposes are not within the scope of the journal. Additionally, disciplines such as soil science, polymer science, and metallurgy fall outside the purview of Separation and Purification Technology. Join us in advancing the field of separation and purification methods for sustainable solutions in chemical and environmental engineering.
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