Ultra-sensitive, fast response microcapsule structure capacitive sensor with encapsulated columnar nano-ZnO for electronic skin

IF 5.8 2区 材料科学 Q2 CHEMISTRY, PHYSICAL
Jie Chen, Lizhu Guan, Minghui Xu, Tianyu Hu, Zhichao Pang, Dongming Shi, Weiyu Wang
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Abstract

The capacitive pressure sensor holds broad prospects in medical devices and electronic skins. However, challenges persist in enhancing the stability of its capacitance and its response/relaxation time. To tackle these issues, we have proposed a highly sensitive capacitive sensor based on polyvinylidene fluoride-trifluoroethylene (P(VDF-TrFE)) with a microcapsule structure coated with nano-ZnO. The sensor integrates a semiconductor filler within a porous microstructure, enabling it to be positioned within the matrix’s pores for the purpose of monitoring human health. This P(VDF-TrFE)-ZnO dielectric layer with a short rod-like ZnO particle-in-micropore (SRP-MP) structure effectively enhances the structural stability and capacitance change rate of the dielectric layer. It boasts an ultrahigh sensitivity of 3.1 kPa-1, a broad pressure range of up to 50 kPa, an ultra-low relaxation response time of 23 ms, and the ability to detect an ultra-low minimum pressure of 50 Pa. The sensor’s structural stability has been significantly improved, and it has demonstrated excellent fatigue resistance in 10,000 cycles tests. Following this, we delved into the sensor’s sensing mechanism. To elucidate the reasons behind the sensor’s enhanced performance, we modeled its interior and conducted finite element analysis simulations (COMSOL) to investigate its internal sensing mechanism and piezoelectric response. Finally, we conducted various tests on the sensor’s human application to clarify its performance in actual situations, demonstrating significant application potential.
用于电子皮肤的封装柱状纳米氧化锌的超灵敏、快速响应微胶囊结构电容式传感器
电容式压力传感器在医疗器械、电子皮肤等领域具有广阔的应用前景。然而,在提高其电容稳定性和响应/弛豫时间方面仍然存在挑战。为了解决这些问题,我们提出了一种基于聚偏氟乙烯-三氟乙烯(P(VDF-TrFE))的高灵敏度电容式传感器,该传感器具有涂有纳米zno的微胶囊结构。该传感器在多孔微结构中集成了半导体填充物,使其能够定位在基质的孔隙中,以监测人体健康。该P(VDF-TrFE)-ZnO介质层具有短棒状的ZnO颗粒微孔(SRP-MP)结构,有效地提高了介质层的结构稳定性和电容变化率。它具有3.1 kPa-1的超高灵敏度,高达50 kPa的宽压力范围,23 ms的超低松弛响应时间,以及检测50 Pa的超低最低压力的能力。该传感器的结构稳定性得到了显著提高,并在10,000次循环试验中表现出优异的抗疲劳性能。在此之后,我们深入研究了传感器的传感机制。为了阐明传感器性能增强背后的原因,我们对其内部进行了建模并进行了有限元分析仿真(COMSOL),以研究其内部传感机制和压电响应。最后,我们对传感器的人体应用进行了各种测试,以阐明其在实际情况下的性能,显示出巨大的应用潜力。
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来源期刊
Journal of Alloys and Compounds
Journal of Alloys and Compounds 工程技术-材料科学:综合
CiteScore
11.10
自引率
14.50%
发文量
5146
审稿时长
67 days
期刊介绍: The Journal of Alloys and Compounds is intended to serve as an international medium for the publication of work on solid materials comprising compounds as well as alloys. Its great strength lies in the diversity of discipline which it encompasses, drawing together results from materials science, solid-state chemistry and physics.
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polydimethylsiloxane (PDMS)
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