Conductive Hydrogel with Ta4C3TX MXene to Detect Human Movement

IF 5.3 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Fan Wu, Long Yu, Liyi Zhou, Jiarong Zhang, Ya’nan Zhao, Chunna Yu, Chang Zhao and Guangjian Xing*, 
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Abstract

Nanocomposite hydrogels with exceptional mechanical properties and sensing performance are ideal for flexible sensors designed to detect human movements and monitor human health. In this study, a composite hydrogel was prepared through in situ polymerization using a combination of poly(methacrylic acid-co-acrylamide) (P(MAA-co-AAM)), poly(3,4-ethylenedioxythiophene)/poly(styrenesulfonate) (PEDOT/PSS), and Ta4C3TX MXene. The resulting P(MAA-co-AAM)/PEDOT/PSS/Ta4C3TX hydrogel features a porous network structure closely cross-linked with hydrogen bonds, providing superior mechanical properties such as high elastic modulus, compressive strength, and low hysteresis ratio. The compressive strength of the hydrogel reaches 386.80 kPa, significantly surpassing that of pure P(MAA-co-AAM) hydrogels and other hydrogels. The piezoresistive sensor developed with this hydrogel demonstrates outstanding pressure sensing capabilities: a sensitivity of 0.44 kPa–1, a low detection limit of 38.63 Pa, a rapid response time of 44 ms, and a recovery time of 58 ms. Notably, the sensor can sustain over 1000 sensing cycles with remarkable stability and weather resistance. It can accurately detect human body movements, such as joint movements, and even recognize subtle facial microexpressions. Furthermore, the sensor can wirelessly monitor robotic movements through a Bluetooth system and accompanying software. This mechanically robust hydrogel holds significant promise for applications in pressure sensors, human-machine interaction, and portable wearable devices.

Abstract Image

Ta4C3TX MXene导电水凝胶检测人体运动
纳米复合水凝胶具有优异的机械性能和传感性能,是设计用于检测人体运动和监测人体健康的柔性传感器的理想选择。本研究以聚(甲基丙烯酸-共丙烯酰胺)(P(MAA-co-AAM))、聚(3,4-乙烯二氧噻吩)/聚(苯乙烯磺酸)(PEDOT/PSS)和Ta4C3TX MXene为原料,通过原位聚合法制备了复合水凝胶。制备的P(MAA-co-AAM)/PEDOT/PSS/Ta4C3TX水凝胶具有与氢键紧密交联的多孔网络结构,具有高弹性模量、抗压强度和低迟滞比等优异的力学性能。水凝胶的抗压强度达到386.80 kPa,明显超过纯P(MAA-co-AAM)水凝胶和其他水凝胶。用该水凝胶开发的压阻式传感器具有出色的压力传感能力:灵敏度为0.44 kPa-1,低检测限为38.63 Pa,快速响应时间为44 ms,恢复时间为58 ms。值得注意的是,该传感器可以维持1000多个传感周期,具有卓越的稳定性和耐候性。它可以准确地检测人体运动,如关节运动,甚至可以识别细微的面部微表情。此外,传感器可以通过蓝牙系统和配套软件无线监控机器人的运动。这种机械坚固的水凝胶在压力传感器、人机交互和便携式可穿戴设备中具有重要的应用前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
CiteScore
8.30
自引率
3.40%
发文量
1601
期刊介绍: ACS Applied Nano Materials is an interdisciplinary journal publishing original research covering all aspects of engineering, chemistry, physics and biology relevant to applications of nanomaterials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important applications of nanomaterials.
文献相关原料
公司名称
产品信息
麦克林
PEDOT:PSS
阿拉丁
Ammonium persulfate (APS)
阿拉丁
N,N'-methylene diacrylamide
阿拉丁
Acrylamide (AAM)
阿拉丁
Tetramethylammonium hydroxide pentahydrate (TMAH)
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