Hongchi Yao, Jing Luo, Yong Xu, Hongtao Liu and Jiguo Tang*,
{"title":"Bubble Formation from a Submerged Microcapillary Nozzle in Novec 649","authors":"Hongchi Yao, Jing Luo, Yong Xu, Hongtao Liu and Jiguo Tang*, ","doi":"10.1021/acs.iecr.4c0339110.1021/acs.iecr.4c03391","DOIUrl":null,"url":null,"abstract":"<p >Bubble formation in liquids is ubiquitous in nature and in various industrial processes, playing a crucial role in water electrolysis, chemical reaction, and boiling. This study investigates bubble formation from submerged microcapillary nozzles in Novec 649, an advanced dielectric fluid with a low global warming potential and toxicity. The behaviors and detachment parameters of the bubbles are analyzed under various gas flow rates and nozzle diameters. We create a bubbling regime map for bubble formation in Novec 649 and develop a scaling law to predict the transition from bubbling without coalescence to bubbling with coalescence by using Weber and Bond numbers. Force analysis reveals that in Novec 649, drag and liquid inertia forces are more significant in bubble detachment compared to bubble formation in water, attributed to its higher density and lower surface tension. Additionally, we develop a new force balance model and a new explicit approximate model to predict the bubble detachment diameter in Novec 649, considering the impact of the waiting time and liquid velocity around the bubble. These models outperform previous models for the experimental data of Novec 649. This study contributes to enhancing our understanding of the dynamics of bubble formation in novel liquids.</p>","PeriodicalId":39,"journal":{"name":"Industrial & Engineering Chemistry Research","volume":"63 50","pages":"22166–22176 22166–22176"},"PeriodicalIF":3.8000,"publicationDate":"2024-12-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Industrial & Engineering Chemistry Research","FirstCategoryId":"5","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.iecr.4c03391","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Bubble formation in liquids is ubiquitous in nature and in various industrial processes, playing a crucial role in water electrolysis, chemical reaction, and boiling. This study investigates bubble formation from submerged microcapillary nozzles in Novec 649, an advanced dielectric fluid with a low global warming potential and toxicity. The behaviors and detachment parameters of the bubbles are analyzed under various gas flow rates and nozzle diameters. We create a bubbling regime map for bubble formation in Novec 649 and develop a scaling law to predict the transition from bubbling without coalescence to bubbling with coalescence by using Weber and Bond numbers. Force analysis reveals that in Novec 649, drag and liquid inertia forces are more significant in bubble detachment compared to bubble formation in water, attributed to its higher density and lower surface tension. Additionally, we develop a new force balance model and a new explicit approximate model to predict the bubble detachment diameter in Novec 649, considering the impact of the waiting time and liquid velocity around the bubble. These models outperform previous models for the experimental data of Novec 649. This study contributes to enhancing our understanding of the dynamics of bubble formation in novel liquids.
期刊介绍:
ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.