{"title":"Deep Learning-Assisted Analysis of GO-Reinforcing Effects on the Interfacial Transition Zone of CWRB.","authors":"Jiajian Yu, Zhiwei Chen, Xiaoli Xu, Xinjie Su, Shuai Liang, Yanchao Wang, Junqing Hong, Shaofeng Zhang","doi":"10.3390/ma17235926","DOIUrl":null,"url":null,"abstract":"<p><p>Understanding the enhancing mechanisms of graphene oxide (GO) on the pore structure characteristics in the interfacial transition zone (ITZ) plays a crucial role in cemented waste rock backfill (CWRB) nanoreinforcement. In the present work, an innovative method based on metal intrusion techniques, backscattered electron (BSE) images, and deep learning is proposed to analyze the micro/nanoscale characteristics of microstructures in the GO-enhanced ITZ. The results showed that the addition of GO reduced the interpore connectivity and the porosity at different pore throats by 53.5-53.8%. GO promotes hydration reaction in the ITZ region; reduces pore circularity, solidity, and aspect ratio; enhances the mechanical strength of CWRB; and reduces transport performance to form a dense microstructure in the ITZ. Deep learning-based analyses were then proposed to classify and recognize BSE image features, with a high average recognition accuracy of 95.8%. After that, the deep Taylor decomposition (DTD) algorithm successfully located the enhanced features of graphene oxide modification in the ITZ. The calculation and verification of the typical pore optimization area of the location show that the optimization efficiency reaches 9.6-9.8%. This study not only demonstrated the deepening of the enhancement effect of GO on the pore structure in cement composites and provided new insights for the structural modification application of GO but also revealed the application prospect of GO in the strengthening of CWRB composites and solid waste recycling.</p>","PeriodicalId":18281,"journal":{"name":"Materials","volume":"17 23","pages":""},"PeriodicalIF":3.1000,"publicationDate":"2024-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11643210/pdf/","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.3390/ma17235926","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Understanding the enhancing mechanisms of graphene oxide (GO) on the pore structure characteristics in the interfacial transition zone (ITZ) plays a crucial role in cemented waste rock backfill (CWRB) nanoreinforcement. In the present work, an innovative method based on metal intrusion techniques, backscattered electron (BSE) images, and deep learning is proposed to analyze the micro/nanoscale characteristics of microstructures in the GO-enhanced ITZ. The results showed that the addition of GO reduced the interpore connectivity and the porosity at different pore throats by 53.5-53.8%. GO promotes hydration reaction in the ITZ region; reduces pore circularity, solidity, and aspect ratio; enhances the mechanical strength of CWRB; and reduces transport performance to form a dense microstructure in the ITZ. Deep learning-based analyses were then proposed to classify and recognize BSE image features, with a high average recognition accuracy of 95.8%. After that, the deep Taylor decomposition (DTD) algorithm successfully located the enhanced features of graphene oxide modification in the ITZ. The calculation and verification of the typical pore optimization area of the location show that the optimization efficiency reaches 9.6-9.8%. This study not only demonstrated the deepening of the enhancement effect of GO on the pore structure in cement composites and provided new insights for the structural modification application of GO but also revealed the application prospect of GO in the strengthening of CWRB composites and solid waste recycling.
期刊介绍:
Materials (ISSN 1996-1944) is an open access journal of related scientific research and technology development. It publishes reviews, regular research papers (articles) and short communications. Our aim is to encourage scientists to publish their experimental and theoretical results in as much detail as possible. Therefore, there is no restriction on the length of the papers. The full experimental details must be provided so that the results can be reproduced. Materials provides a forum for publishing papers which advance the in-depth understanding of the relationship between the structure, the properties or the functions of all kinds of materials. Chemical syntheses, chemical structures and mechanical, chemical, electronic, magnetic and optical properties and various applications will be considered.