Two-Dimensional Transition Metal Dichalcogenides (2D TMDs) Coupled With Zero-Dimensional Nanomaterials (0D NMs) for Advanced Photodetection.

Abstract

The integration of 2D transition metal dichalcogenides (TMDs) with other materials presents a promising approach to overcome inherent limitations and enable the development of novel functionalities. In particular, 0D nanomaterials (0D NMs) offer notable advantages for photodetection, including broadband light absorption, size-dependent optoelectronic properties, high quantum efficiency, and good compatibility. Herein, the integration of 0D NMs with 2D TMDs to develop high-performance photodetectors is reviewed. The review provides a comprehensive overview of different types of 0D NMs, including plasma nanoparticles (NPs), up-conversion NPs, quantum dots (QDs), nanocrystals (NCs), and small molecules. The discussion starts with an analysis of the mechanism of 0D NMs on 2D TMDs in photodetection, exploring various strategies for improving the performance of hybrid 2D TMDs/0D NMs. Recent advancements in photodetectors combining 2D TMDs with 0D NMs are investigated, particularly emphasizing critical factors such as photosensitivity, photogain, specific detectivity, and photoresponse speed. The review concludes with a summary of the current status, highlighting the existing challenges and prospective developments in the advancement of 0D NMs/2D TMDs-based photodetectors.