Concurrently Boosting Activity and Stability of Oxygen Reduction Reaction Catalysts via Judiciously Crafting Fe–Mn Dual Atoms for Fuel Cells

IF 26.6 1区 材料科学 Q1 Engineering
Lei Zhang, Yuchen Dong, Lubing Li, Yuchuan Shi, Yan Zhang, Liting Wei, Chung-Li Dong, Zhiqun Lin, Jinzhan Su
{"title":"Concurrently Boosting Activity and Stability of Oxygen Reduction Reaction Catalysts via Judiciously Crafting Fe–Mn Dual Atoms for Fuel Cells","authors":"Lei Zhang,&nbsp;Yuchen Dong,&nbsp;Lubing Li,&nbsp;Yuchuan Shi,&nbsp;Yan Zhang,&nbsp;Liting Wei,&nbsp;Chung-Li Dong,&nbsp;Zhiqun Lin,&nbsp;Jinzhan Su","doi":"10.1007/s40820-024-01580-5","DOIUrl":null,"url":null,"abstract":"<div><h2>Highlights</h2><div>\n \n <ul>\n <li>\n <p>Fe–Mn dual-atom catalysts exhibit superior oxygen reduction reaction (ORR) activity and stability, with high half-wave potentials in both alkaline and acidic conditions.</p>\n </li>\n <li>\n <p>Synergistic Mn incorporation effectively anchors Fe atoms, mitigates the Fenton reaction, and enhances the durability of ORR catalysts.</p>\n </li>\n <li>\n <p>Advanced characterization and density-functional theory calculations reveal Mn-induced electronic structure modifications, promoting superior ORR kinetics and active site performance.</p>\n </li>\n <li>\n <p>(FeMn-DA)-N-C catalysts show remarkable potential for practical fuel cell applications.</p>\n </li>\n </ul>\n </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6000,"publicationDate":"2024-12-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01580-5.pdf","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano-Micro Letters","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s40820-024-01580-5","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Engineering","Score":null,"Total":0}
引用次数: 0

Abstract

Highlights

  • Fe–Mn dual-atom catalysts exhibit superior oxygen reduction reaction (ORR) activity and stability, with high half-wave potentials in both alkaline and acidic conditions.

  • Synergistic Mn incorporation effectively anchors Fe atoms, mitigates the Fenton reaction, and enhances the durability of ORR catalysts.

  • Advanced characterization and density-functional theory calculations reveal Mn-induced electronic structure modifications, promoting superior ORR kinetics and active site performance.

  • (FeMn-DA)-N-C catalysts show remarkable potential for practical fuel cell applications.

先进的表征和密度泛函理论计算揭示了锰诱导的电子结构修饰,促进了卓越的 ORR 动力学和活性位点性能。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Nano-Micro Letters
Nano-Micro Letters NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
32.60
自引率
4.90%
发文量
981
审稿时长
1.1 months
期刊介绍: Nano-Micro Letters is a peer-reviewed, international, interdisciplinary, and open-access journal published under the SpringerOpen brand. Nano-Micro Letters focuses on the science, experiments, engineering, technologies, and applications of nano- or microscale structures and systems in various fields such as physics, chemistry, biology, material science, and pharmacy.It also explores the expanding interfaces between these fields. Nano-Micro Letters particularly emphasizes the bottom-up approach in the length scale from nano to micro. This approach is crucial for achieving industrial applications in nanotechnology, as it involves the assembly, modification, and control of nanostructures on a microscale.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信