Polariton-Induced Transparency in Multiple Quantum Wells Probed by Time Domain Brillouin Scattering

IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Marek Karzel, Anton K. Samusev, Tetiana L. Linnik, Mario Littmann, Dirk Reuter, Manfred Bayer, Alexey V. Scherbakov, Andrey V. Akimov
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Abstract

The interference of the incident light reflected from the surface of a medium and from a picosecond strain pulse propagating through it results in temporal oscillations of the reflected intensity. This phenomenon, called time-domain Brillouin scattering, enables us to gain information about the optical field inside the medium. The oscillation amplitude decreases with increase of the distance from the strain pulse to the surface if the incident light is strongly absorbed, while it remains constant if the medium is transparent. Here we exploit time domain Brillouin scattering to probe the optical field inside a multiple quantum well layer for light strongly coupling to excitons and forming polaritons. At low excitation density, we observe conventional Brillouin oscillations whose amplitude is small when the strain pulse is positioned far from the surface due to the strong absorption of polaritons in the vicinity of the exciton resonance. At elevated optical density, the absorption disappears, the medium becomes transparent, and the amplitude of the oscillations does not depend on the distance of the strain pulse from the surface. We explain this effect of polariton-induced transparency by the increase of the incoherent exciton density generated as result of polariton scattering. Finally, the increase of the exciton density leads to transition of the exciton gas to a collective state, resulting in collapse of the polariton state and propagation of the incident light in the medium without absorption.

Abstract Image

用时域布里渊散射探测多量子阱中的极化诱导透明
从介质表面反射的入射光和通过介质传播的皮秒应变脉冲的干涉导致反射强度的时间振荡。这种现象被称为时域布里渊散射,它使我们能够获得有关介质内部光场的信息。当入射光被强吸收时,振荡幅度随应变脉冲到表面距离的增加而减小,而当介质为透明时,振荡幅度保持不变。在这里,我们利用时域布里渊散射来探测光与激子强耦合并形成极化的多量子阱层内的光场。在低激发密度下,由于激子共振附近极化子的强烈吸收,当应变脉冲位于远离表面时,我们观察到常规布里渊振荡的振幅很小。当光密度升高时,吸收消失,介质变得透明,振荡幅度不依赖于应变脉冲与表面的距离。我们通过极化子散射产生的非相干激子密度的增加来解释极化子诱导透明度的这种效应。最后,激子密度的增加导致激子气体跃迁到集体态,导致极化态坍缩,入射光在介质中传播而不被吸收。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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