Illuminating for purity: photocatalytic and photothermal membranes for sustainable oil-water separation

IF 11.4 1区环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL

Water Research Pub Date : 2024-12-08 DOI:10.1016/j.watres.2024.122919

Hongyuan Zhu, Zhenyu Guo, Wei Yu, Shasha Yuan, Liguo Shen, Die Ling Zhao, Hongjun Lin

{"title":"Illuminating for purity: photocatalytic and photothermal membranes for sustainable oil-water separation","authors":"Hongyuan Zhu, Zhenyu Guo, Wei Yu, Shasha Yuan, Liguo Shen, Die Ling Zhao, Hongjun Lin","doi":"10.1016/j.watres.2024.122919","DOIUrl":null,"url":null,"abstract":"The integration of photocatalytic and photothermal materials with oil-water separation membranes marks a significant advancement in sustainable separation technologies. These hybrid membranes exhibit exceptional functionalities, including resistance to oil fouling, self-cleaning, antibacterial properties, and reduced oil viscosity. Based on their reaction mechanisms, current photocatalytic and photothermal membranes are categorized into four types, i.e., photocatalytic membranes, photo-Fenton membranes, PMS-assisted photocatalytic membranes, and photothermal membranes. Under light irradiation, photocatalytically functionalized membranes generate reactive oxygen species (ROS) that degrade organic pollutants and inactivate bacteria on the membrane surfaces, enabling in-situ cleaning and regeneration. In addition to the above benefits, photothermal membranes achieve reduction of oil viscosity for higher membrane permeation and removal of light oil from membrane surfaces through light-induced heating. This review first explores the mechanisms underlying light-driven advanced oxidation processes (AOPs) and photothermal effects, followed by an in-depth discussion on the fabrication methods of these membranes. Additionally, the applications of photocatalytic and photothermal membranes in oil-water separation are examined, with an emphasis on how the photocatalytic and photothermal materials contribute to membrane functionality. Finally, this review presents the challenges currently faced by photocatalytic and photothermal membranes and outlines future research directions.","PeriodicalId":443,"journal":{"name":"Water Research","volume":"113 1","pages":""},"PeriodicalIF":11.4000,"publicationDate":"2024-12-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Water Research","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.watres.2024.122919","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}

引用次数: 0

Abstract

The integration of photocatalytic and photothermal materials with oil-water separation membranes marks a significant advancement in sustainable separation technologies. These hybrid membranes exhibit exceptional functionalities, including resistance to oil fouling, self-cleaning, antibacterial properties, and reduced oil viscosity. Based on their reaction mechanisms, current photocatalytic and photothermal membranes are categorized into four types, i.e., photocatalytic membranes, photo-Fenton membranes, PMS-assisted photocatalytic membranes, and photothermal membranes. Under light irradiation, photocatalytically functionalized membranes generate reactive oxygen species (ROS) that degrade organic pollutants and inactivate bacteria on the membrane surfaces, enabling in-situ cleaning and regeneration. In addition to the above benefits, photothermal membranes achieve reduction of oil viscosity for higher membrane permeation and removal of light oil from membrane surfaces through light-induced heating. This review first explores the mechanisms underlying light-driven advanced oxidation processes (AOPs) and photothermal effects, followed by an in-depth discussion on the fabrication methods of these membranes. Additionally, the applications of photocatalytic and photothermal membranes in oil-water separation are examined, with an emphasis on how the photocatalytic and photothermal materials contribute to membrane functionality. Finally, this review presents the challenges currently faced by photocatalytic and photothermal membranes and outlines future research directions.

Abstract Image

查看原文本刊更多论文

求助全文

约1分钟内获得全文求助全文

来源期刊

Water Research 环境科学-工程：环境

CiteScore

20.80

自引率

9.40%

发文量

1307

审稿时长

38 days

期刊介绍： Water Research, along with its open access companion journal Water Research X, serves as a platform for publishing original research papers covering various aspects of the science and technology related to the anthropogenic water cycle, water quality, and its management worldwide. The audience targeted by the journal comprises biologists, chemical engineers, chemists, civil engineers, environmental engineers, limnologists, and microbiologists. The scope of the journal include: •Treatment processes for water and wastewaters (municipal, agricultural, industrial, and on-site treatment), including resource recovery and residuals management; •Urban hydrology including sewer systems, stormwater management, and green infrastructure; •Drinking water treatment and distribution; •Potable and non-potable water reuse; •Sanitation, public health, and risk assessment; •Anaerobic digestion, solid and hazardous waste management, including source characterization and the effects and control of leachates and gaseous emissions; •Contaminants (chemical, microbial, anthropogenic particles such as nanoparticles or microplastics) and related water quality sensing, monitoring, fate, and assessment; •Anthropogenic impacts on inland, tidal, coastal and urban waters, focusing on surface and ground waters, and point and non-point sources of pollution; •Environmental restoration, linked to surface water, groundwater and groundwater remediation; •Analysis of the interfaces between sediments and water, and between water and atmosphere, focusing specifically on anthropogenic impacts; •Mathematical modelling, systems analysis, machine learning, and beneficial use of big data related to the anthropogenic water cycle; •Socio-economic, policy, and regulations studies.