{"title":"Quantum Efficiency and Vertical Position of Quantum Emitters in hBN Determined by Purcell Effect in Hybrid Metal-Dielectric Planar Photonic Structures","authors":"Domitille Gérard, Aurélie Pierret, Helmi Fartas, Bruno Berini, Stéphanie Buil, Jean-Pierre Hermier, Aymeric Delteil","doi":"10.1021/acsphotonics.4c01416","DOIUrl":null,"url":null,"abstract":"Color centers in hexagonal boron nitride (hBN) advantageously combine excellent photophysical properties with the potential for integration in highly compact devices. Progress toward scalable integration necessitates a high quantum efficiency and an efficient photon collection. In this context, we compare the optical characteristics of individual hBN color centers generated by electron irradiation in two different electromagnetic environments. We keep track of well-identified emitters that we characterize before and after the dry transfer of exfoliated crystals. This comparison provides information about their quantum efficiency, which we find close to unity, as well as their vertical position in the crystal with nanometric precision, which we find away from the flake surfaces. Our work suggests hybrid dielectric-metal planar structures as an efficient tool for characterizing quantum emitters in addition to improving the count rate and can be generalized to other emitters in 2D materials or in planar photonic structures.","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"17 1","pages":""},"PeriodicalIF":6.5000,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Photonics","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1021/acsphotonics.4c01416","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Color centers in hexagonal boron nitride (hBN) advantageously combine excellent photophysical properties with the potential for integration in highly compact devices. Progress toward scalable integration necessitates a high quantum efficiency and an efficient photon collection. In this context, we compare the optical characteristics of individual hBN color centers generated by electron irradiation in two different electromagnetic environments. We keep track of well-identified emitters that we characterize before and after the dry transfer of exfoliated crystals. This comparison provides information about their quantum efficiency, which we find close to unity, as well as their vertical position in the crystal with nanometric precision, which we find away from the flake surfaces. Our work suggests hybrid dielectric-metal planar structures as an efficient tool for characterizing quantum emitters in addition to improving the count rate and can be generalized to other emitters in 2D materials or in planar photonic structures.
期刊介绍:
Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.