{"title":"Time-series observation of 210Pb sinking fluxes in the western North Pacific","authors":"Hajime Kawakami","doi":"10.1007/s10967-024-09801-2","DOIUrl":null,"url":null,"abstract":"<div><p>We observed the lead-210 (<sup>210</sup>Pb) sinking flux in subarctic and subtropical regions of the western North Pacific Ocean over time. The <sup>210</sup>Pb fluxes in the mesopelagic and bathypelagic zones were estimated from the disequilibrium between <sup>210</sup>Pb and radium-226 (<sup>226</sup>Ra) in the water column over the 4 seasons during several years. In the subarctic region, <sup>210</sup>Pb fluxes were larger (28–29 dpm m<sup>–2</sup> d<sup>–1</sup> at 500 m; 68–70 dpm m<sup>–2</sup> d<sup>–1</sup> at 4810 m) than those in the subtropical region (22–24 dpm m<sup>–2</sup> d<sup>–1</sup> at 500 m; 46–49 dpm m<sup>–2</sup> d<sup>–1</sup> at 4810 m). These results imply that the strength of the biological pump in the mesopelagic and bathypelagic zones is larger in the subarctic region than in the subtropical region of the western North Pacific. We also determined <sup>210</sup>Pb in sinking particles collected by moored sediment traps. In the subarctic (subtropical) region, the annual average of trapped <sup>210</sup>Pb flux at 500 and 4810 m were 3.0 (4.6) and 24.2 (18.6) dpm m<sup>–2</sup> d<sup>–1</sup>, respectively. Estimated from the <sup>210</sup>Pb flux in the water column and the <sup>210</sup>Pb flux in the sinking particles in the sediment trap experiment, the trapping efficiencies at 500 m (10–20%) were about a half of those at 4810 m (35–40%) in the sediment trap experiment.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"333 12","pages":"6507 - 6514"},"PeriodicalIF":1.5000,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Radioanalytical and Nuclear Chemistry","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1007/s10967-024-09801-2","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
引用次数: 0
Abstract
We observed the lead-210 (210Pb) sinking flux in subarctic and subtropical regions of the western North Pacific Ocean over time. The 210Pb fluxes in the mesopelagic and bathypelagic zones were estimated from the disequilibrium between 210Pb and radium-226 (226Ra) in the water column over the 4 seasons during several years. In the subarctic region, 210Pb fluxes were larger (28–29 dpm m–2 d–1 at 500 m; 68–70 dpm m–2 d–1 at 4810 m) than those in the subtropical region (22–24 dpm m–2 d–1 at 500 m; 46–49 dpm m–2 d–1 at 4810 m). These results imply that the strength of the biological pump in the mesopelagic and bathypelagic zones is larger in the subarctic region than in the subtropical region of the western North Pacific. We also determined 210Pb in sinking particles collected by moored sediment traps. In the subarctic (subtropical) region, the annual average of trapped 210Pb flux at 500 and 4810 m were 3.0 (4.6) and 24.2 (18.6) dpm m–2 d–1, respectively. Estimated from the 210Pb flux in the water column and the 210Pb flux in the sinking particles in the sediment trap experiment, the trapping efficiencies at 500 m (10–20%) were about a half of those at 4810 m (35–40%) in the sediment trap experiment.
期刊介绍:
An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.