{"title":"Electrophoretically deposited graphene oxide/molybdenum disulfide composite on quartz crystal microbalance for ethyl acetate VOC detection","authors":"Wei Yin Lim, Choon-Hian Goh, Keenan Zhihong Yap, Narayanan Ramakrishnan","doi":"10.1007/s10853-024-10465-2","DOIUrl":null,"url":null,"abstract":"<div><p>The presence of volatile organic compounds (VOCs) poses significant risks to air quality and human health. However, the existing sensing technologies encounter limitations in efficient sensors fabrication. Techniques like spin coating and drop casting offer rapid deposition, but lack precise control, while layer-by-layer assembly provides superior control but is time-consuming. To address this gap, this study employed electrophoretic deposition (EPD) techniques to rapidly coat graphene oxide (GO)/molybdenum disulfide (MoS<sub>2</sub>) composite on Quartz Crystal Microbalance (QCM) sensors. Various ratios of GO/MoS<sub>2</sub> composites (e.g., GO/MoS<sub>2</sub>_1, GO/MoS<sub>2</sub>_2, and GO/MoS<sub>2</sub>_3), as well as GO and MoS<sub>2</sub> alone were tested to assess their gas sensing capabilities. The GO/MoS<sub>2</sub>_2 composite exhibited a 78% increase in sensitivity to ethyl acetate over other coatings. Surface characterization techniques, including FESEM, EDX, XPS, and Raman spectroscopy, were used to confirm the composite’ structure, and the sensing mechanisms involving adsorption and desorption were discussed. These findings highlight the potential of GO/MoS<sub>2</sub> composites for enhancing VOC detection in gas sensing applications.</p><h3>Graphical Abstract</h3><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":645,"journal":{"name":"Journal of Materials Science","volume":"59 46","pages":"21277 - 21293"},"PeriodicalIF":3.5000,"publicationDate":"2024-11-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Materials Science","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s10853-024-10465-2","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The presence of volatile organic compounds (VOCs) poses significant risks to air quality and human health. However, the existing sensing technologies encounter limitations in efficient sensors fabrication. Techniques like spin coating and drop casting offer rapid deposition, but lack precise control, while layer-by-layer assembly provides superior control but is time-consuming. To address this gap, this study employed electrophoretic deposition (EPD) techniques to rapidly coat graphene oxide (GO)/molybdenum disulfide (MoS2) composite on Quartz Crystal Microbalance (QCM) sensors. Various ratios of GO/MoS2 composites (e.g., GO/MoS2_1, GO/MoS2_2, and GO/MoS2_3), as well as GO and MoS2 alone were tested to assess their gas sensing capabilities. The GO/MoS2_2 composite exhibited a 78% increase in sensitivity to ethyl acetate over other coatings. Surface characterization techniques, including FESEM, EDX, XPS, and Raman spectroscopy, were used to confirm the composite’ structure, and the sensing mechanisms involving adsorption and desorption were discussed. These findings highlight the potential of GO/MoS2 composites for enhancing VOC detection in gas sensing applications.
期刊介绍:
The Journal of Materials Science publishes reviews, full-length papers, and short Communications recording original research results on, or techniques for studying the relationship between structure, properties, and uses of materials. The subjects are seen from international and interdisciplinary perspectives covering areas including metals, ceramics, glasses, polymers, electrical materials, composite materials, fibers, nanostructured materials, nanocomposites, and biological and biomedical materials. The Journal of Materials Science is now firmly established as the leading source of primary communication for scientists investigating the structure and properties of all engineering materials.