Evidencing Dissipation Dilution in Large-Scale Arrays of Single-Layer WSe2 Mechanical Resonators

IF 4.3 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC
Michael Pitts, Matthew Feuer, Anthony K. C. Tan, Alejandro R.-P. Montblanch, James Kerfoot, Evgeny M. Alexeev, Michael Högen, Patrick Hays, Seth A. Tongay, Andrea C. Ferrari, Mete Atatüre and Dhiren M. Kara*, 
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Abstract

Micromechanical resonators with very low mass are highly desirable for sensing and transduction applications. Layered materials (LMs) can be used to fabricate single- to few-atom thick suspended membranes, representing the ultimate limit to low mass. Transition-metal dichalcogenides (TMDs), such as WSe2, are particularly compelling because they can host spatially confined excitons in single layer (1L), potentially enabling the creation of nonclassical mechanical states and interconnects between quantum networks and processors. However, these exciting prospects have been tempered by low device yields, invasive methods for detecting resonator motion, and high mechanical damping. Here, we report the creation of mechanical resonators by suspending 1L-WSe2 across a 90 × 90 array of 2.5-μm diameter holes with a > 75% success rate. We detect the resonator room-temperature (RT) Brownian motion and measure resonator mass to quantify contamination, using below-bandgap laser interferometry. We investigate the relation between frequency, diameter, and mechanical quality factor, which can exceed 1000 in our devices. We find the dependence agrees with the effect of dissipation dilution, highlighting the importance of reducing mechanical mode-bending. Key to this is the large-scale, high-quality arrays that make it possible to access a frequency range that surpasses previous works. Further, the ability to fabricate large numbers of 1L resonators, and the simplicity of probing their motion without electrodes or an underlying reflective substrate, facilitates previously hard-to-reach configurations, such as resonators in phononic crystals or within optical cavities.

Abstract Image

单层 WSe2 机械谐振器大规模阵列中的耗散稀释证明
对于传感和传导应用来说,质量极低的微型机械谐振器是非常理想的。层状材料(LMs)可用于制造单原子到几原子厚的悬浮膜,这代表了低质量的终极极限。二卤化过渡金属(TMD),如 WSe2,尤其引人注目,因为它们可以在单层(1L)中容纳空间约束激子,从而有可能创造出非经典的机械状态以及量子网络和处理器之间的互连。然而,这些令人兴奋的前景却因器件产量低、检测谐振器运动的侵入性方法以及高机械阻尼而受到了影响。在这里,我们报告了通过在 90 × 90 直径为 2.5 微米的孔阵列上悬挂 1L-WSe2 来创建机械谐振器的情况,成功率为 75%。我们利用带隙以下激光干涉测量法检测谐振器的室温布朗运动,并测量谐振器质量以量化污染。我们研究了频率、直径和机械品质因数(在我们的设备中可能超过 1000)之间的关系。我们发现,这种关系与耗散稀释效应一致,突出了减少机械模式弯曲的重要性。这其中的关键是大规模、高质量的阵列,它使我们有可能获得超越以往工作的频率范围。此外,制造大量 1L 谐振器的能力,以及在没有电极或底层反射基底的情况下探测其运动的简便性,都为以前难以触及的配置提供了便利,例如声子晶体中或光腔内的谐振器。
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来源期刊
CiteScore
7.20
自引率
4.30%
发文量
567
期刊介绍: ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric. Indexed/​Abstracted: Web of Science SCIE Scopus CAS INSPEC Portico
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