Facile synthesis of 3D porous SiCNWs/Ti3C2Tx/RGO composite aerogels with electromagnetic wave absorption and thermal insulation properties

IF 2.8 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY
Xin Cheng, Xingmin Liu, Jijie Wang, Boxiong Zheng, Shaowei Lu, Yutuo Hua, Zhisheng Nong, Yutong Song
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Abstract

At present, the preparation of absorbing materials that combine light weight, ultra-wideband absorption and good thermal insulation performance is still an insurmountable gap. Here, we constructed a three-dimensional porous structure in the hope of obtaining excellent microwave absorption and heat insulation properties. In this paper, a unique three-dimensional porous SiCNWs/Ti3C2Tx/RGO (STR) aerogel was prepared by hydrothermal treatment. When the mass ratio of SiCNWs, Ti3C2Tx and GO is 2:1:1, the effective absorption bandwidth of STR aerogel reaches 8.10 GHz (9.90–18.00 GHz). Moreover, the porous structure can effectively reduce the heat radiation transfer. After heating at 300 ℃ for 1 h, STR aerogel can effectively isolate the temperature of about 160 ℃, which proves that STR has good thermal insulation performance. In addition, the formation mechanism of the STR aerogels and the mechanism of thermal insulation and electromagnetic wave absorption of aerogels are also discussed, which will contribute to the development and application of new lightweight stealth material.

轻松合成具有电磁波吸收和隔热性能的三维多孔 SiCNWs/Ti3C2Tx/RGO 复合气凝胶
目前,制备兼具轻质、超宽带吸收和良好隔热性能的吸收材料仍是一个难以逾越的鸿沟。在此,我们构建了一种三维多孔结构,希望获得优异的微波吸收和隔热性能。本文通过水热处理制备了一种独特的三维多孔 SiCNWs/Ti3C2Tx/RGO (STR) 气凝胶。当 SiCNWs、Ti3C2Tx 和 GO 的质量比为 2:1:1 时,STR 气凝胶的有效吸收带宽达到 8.10 GHz(9.90-18.00 GHz)。此外,多孔结构还能有效降低热辐射传导。在 300 ℃ 下加热 1 h 后,STR 气凝胶能有效隔绝约 160 ℃ 的温度,这证明了 STR 具有良好的隔热性能。此外,还探讨了STR气凝胶的形成机理以及气凝胶的隔热和电磁波吸收机理,这将有助于新型轻质隐身材料的开发和应用。
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来源期刊
Applied Physics A
Applied Physics A 工程技术-材料科学:综合
CiteScore
4.80
自引率
7.40%
发文量
964
审稿时长
38 days
期刊介绍: Applied Physics A publishes experimental and theoretical investigations in applied physics as regular articles, rapid communications, and invited papers. The distinguished 30-member Board of Editors reflects the interdisciplinary approach of the journal and ensures the highest quality of peer review.
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