Unraveling the Nature of Lasing Emission from Hybrid Silicon Nitride and Colloidal Nanocrystal Photonic Crystals with Low Refractive Index Contrast

IF 6.5 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Ivo Tanghe*, Tom Vandekerckhove, Margarita Samoli, Amelia Waters, Dulanjan Harankahage, Mikhail Zamkov, Zeger Hens, Christian Seassal, Hai-Son Nguyen, Dries Van Thourhout and Pieter Geiregat*, 
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Abstract

Silicon nitride is used for its low optical loss and high thermal stability, making it a suitable platform for visible-light applications in integrated photonic devices. However, its application has been limited due to inefficient light emission, a problem addressed by integrating various types of light emitters onto the platform. In particular, the integration of solution-processable colloidal nanocrystals (NCs) as optical gain materials onto the silicon nitride platform is a promising route but requires a more solid theoretical footing. By leveraging 2D surface-emitting photonic crystal structures combined with NCs, we effectively confine and manipulate light to achieve lasing from green to red. Building on this, we model the light–matter interactions of the low index contrast NC/nitride platform, validated by extensive experimental validations through Fourier imaging techniques, revealing the full photonic band structure and showing clear mode congestion. These comprehensive studies confirm the potential of hybrid NC-based structures for fully integrated on-chip laser applications and indicate routes for further improvement.

Abstract Image

揭示具有低折射率对比的混合氮化硅和胶体纳米晶光子晶体的激光发射本质
氮化硅具有低光学损耗和高热稳定性的特点,是集成光子器件中可见光应用的合适平台。然而,由于光发射效率低,氮化硅的应用一直受到限制,这一问题可通过在平台上集成各种类型的光发射器来解决。特别是,将可溶液加工的胶体纳米晶体(NC)作为光学增益材料集成到氮化硅平台上是一条很有前景的途径,但需要更坚实的理论基础。通过利用二维表面发光光子晶体结构与 NCs 的结合,我们有效地限制和操纵了光,实现了从绿色到红色的激光。在此基础上,我们建立了低指数对比数控/氮化物平台的光-物质相互作用模型,并通过傅立叶成像技术进行了广泛的实验验证,揭示了完整的光子带结构并显示出清晰的模式拥塞。这些全面的研究证实了基于混合 NC 结构的全集成片上激光应用的潜力,并指出了进一步改进的途径。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
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