Analytical study of bioclogging effects in underground hydrogen storage

IF 8.1 2区 工程技术 Q1 CHEMISTRY, PHYSICAL
Siqin Yu , Shaowen Mao , Mohamed Mehana
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引用次数: 0

Abstract

Underground hydrogen storage (UHS) in porous formations is emerging as a promising solution to global decarbonization. While much knowledge from geologic carbon sequestration is transferable, a critical technical challenge unique to UHS is the active interaction between hydrogen and microbes. In this study, we develop an analytical framework to quantify the bioclogging effect in saline aquifers at the reservoir scale. Our objective is to understand how bioclogging will impact UHS operations and explore potential mitigation strategies. To achieve this, we extend the Buckley–Leverett solution to construct the solution, which is computationally efficient by preserving the analytical nature. Our findings reveal that near-well permeability impairment could be up to twice as severe as previously estimated, emphasizing the advantages of deeper formations with higher temperatures, where microbial activity is reduced. Furthermore, we observed an increase in hydrogen recovery and a progressive advancement of the gas plume front position across storage cycles. These insights not only contribute to designing operational conditions but also suggest effective mitigation strategies for maximizing hydrogen storage efficiency.
地下储氢中生物积液效应的分析研究
多孔地层中的地下氢储存(UHS)正在成为全球脱碳的一种有前途的解决方案。虽然地质碳封存方面的许多知识都可以借鉴,但氢与微生物之间的积极互动是地下储氢所特有的一项关键技术挑战。在本研究中,我们开发了一个分析框架,用于在储层尺度上量化含盐含水层中的生物积液效应。我们的目标是了解生物积水将如何影响超高压制氢系统的运行,并探索潜在的缓解策略。为此,我们扩展了 Buckley-Leverett 解法来构建解决方案,通过保留分析性质来提高计算效率。我们的研究结果表明,近井渗透率受损的严重程度可能是之前估计的两倍,这就强调了温度较高的深层地层的优势,因为在那里微生物的活动会减少。此外,我们还观察到氢气回收率的提高,以及气体羽流前沿位置在整个存储周期中的逐步推进。这些见解不仅有助于设计运行条件,还提出了有效的缓解策略,以最大限度地提高氢气存储效率。
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来源期刊
International Journal of Hydrogen Energy
International Journal of Hydrogen Energy 工程技术-环境科学
CiteScore
13.50
自引率
25.00%
发文量
3502
审稿时长
60 days
期刊介绍: The objective of the International Journal of Hydrogen Energy is to facilitate the exchange of new ideas, technological advancements, and research findings in the field of Hydrogen Energy among scientists and engineers worldwide. This journal showcases original research, both analytical and experimental, covering various aspects of Hydrogen Energy. These include production, storage, transmission, utilization, enabling technologies, environmental impact, economic considerations, and global perspectives on hydrogen and its carriers such as NH3, CH4, alcohols, etc. The utilization aspect encompasses various methods such as thermochemical (combustion), photochemical, electrochemical (fuel cells), and nuclear conversion of hydrogen, hydrogen isotopes, and hydrogen carriers into thermal, mechanical, and electrical energies. The applications of these energies can be found in transportation (including aerospace), industrial, commercial, and residential sectors.
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