Realization of Z2 Topological Photonic Insulators Made from Multilayer Transition Metal Dichalcogenides.

Abstract

Monolayers of semiconducting transition metal dichalcogenides (TMDs) have long attracted interest for their intriguing optical and electronic properties. Recently, TMDs in their quasi-bulk form have started to show considerable promise for nanophotonics thanks to their high refractive indices, large optical anisotropy, wide transparency windows reaching to the visible, and robust room temperature excitons promising for nonlinear optics. Adherence of TMD layers to any substrate via van der Waals forces is a further key enabler for the nanofabrication of complex photonic structures requiring heterointegration. Here, we use the attractive properties of TMDs and realize topological spin-Hall photonic lattices made of arrays of triangular nanoholes in 50 to 100 nm thick WS₂ flakes exfoliated on SiO₂/Si substrates. High-quality structures are achieved by taking advantage of anisotropic dry etching dictated by the crystal axes of WS₂. Reflectance measurements at room temperature show a photonic gap opening in the near-infrared in trivial and topological phases. Unidirectional propagation along the domain interface is demonstrated in real space via circularly polarized laser excitation in samples with both zigzag and armchair domain boundaries. Finite-difference time-domain simulations are used to interpret optical spectroscopy results. Our work demonstrates the feasibility of more complex nanophotonic devices based on the layered (van der Waals) materials platform.