Quantifying the polar skyrmion motion barrier in an oxide heterostructure

IF 5.8 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Nanoscale Pub Date : 2024-11-12 DOI:10.1039/d4nr03686g
Lizhe Hu, Yuhui Huang, Yong Jun Wu, Zijian Hong
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Abstract

Exotic polar topologies such as polar skyrmions have been widely observed in the ferroelectric superlattice system. The dynamic motion of the polar skyrmion under external forces holds promise for applications in advanced electronic devices such as race-track memory. Meanwhile, the polar skyrmion motion has proven to be challenging due to the strong skyrmion-skyrmion interaction and a lack of a mechanism similar to the spin-transfer torque. In this study, we have developed a nudged elastic band (NEB) method to quantify the polar skyrmion motion barrier along a specific trajectory. It is indicated that the skyrmion motion barrier can be significantly reduced with the reduction of the periodicity to 8 u.c., due to the large reduction of the skyrmion size. Moreover, this barrier can also be greatly reduced with a small external electric potential. Following the analysis, we further performed phase-field simulation to verify the collective motion of the polar skyrmion. We have demonstrated the skyrmion motion by applying a 5 μN mechanical force using a blame-shaped indenter with a periodicity of 8 unit cells, under an external applied voltage of 1.5 V. This study further paves the way for the design of the polar skyrmion-based electronic devices.
量化氧化物异质结构中的极性天电离运动屏障
在铁电超晶格系统中已广泛观察到极性天幕等奇异的极性拓扑结构。极性天幕在外力作用下的动态运动有望应用于赛道存储器等先进电子设备中。与此同时,由于极性天融子与天融子之间存在很强的相互作用,而且缺乏类似于自旋转移力矩的机制,因此极性天融子的运动被证明具有挑战性。在这项研究中,我们开发了一种裸弹带(NEB)方法来量化沿特定轨迹的极性天融运动障碍。结果表明,随着周期性减小到 8 u.c.,天离子运动障碍会显著减小,这是由于天离子尺寸的大幅减小。此外,小的外部电势也能大大降低这一障碍。在分析之后,我们进一步进行了相场模拟,以验证极性天融子的集体运动。在 1.5 V 的外加电压下,我们使用周期为 8 个单元格的责状压头施加了 5 μN 的机械力,证明了天空离子的运动。这项研究为设计基于极性天电离子的电子器件进一步铺平了道路。
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来源期刊
Nanoscale
Nanoscale CHEMISTRY, MULTIDISCIPLINARY-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
12.10
自引率
3.00%
发文量
1628
审稿时长
1.6 months
期刊介绍: Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.
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