Frontiers in metal–organic frameworks: innovative nanomaterials for next-generation supercapacitors

IF 23.2 2区 材料科学 Q1 MATERIALS SCIENCE, COMPOSITES
Mohd Zahid Ansari, Faiza Habib, Jhalak Gupta, Abdullah Saad Alsubaie, Imad Barsoum, Akram Alfantazi, Mudasir A. Yatoo, Zubair Ahmad, Iftikhar Hussain
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Abstract

Metal–organic frameworks (MOFs) have emerged as a versatile class of porous materials with tremendous potential for various applications, including energy storage devices. This review provides a comprehensive analysis of recent advancements and applications of MOFs in the field of energy storage including a brief overview of the fundamental aspects of MOFs, including their synthesis, structural diversity, and tuneable properties. MOFs have been extensively investigated for applications in advanced energy storage systems including supercapacitors. MOFs can be employed as electrode materials, separators, and catalysts, offering enhanced electrochemical performance, improved charge/discharge rates, and prolonged cycling stability. The unique tunability of MOFs allows for the rational design of tailored materials with desired properties, such as high specific capacity, excellent conductivity, and superior cycling stability. The recent developments in MOF-based electrochemical capacitors, particularly the significant progress reported in achieving high energy and power densities, are noteworthy. The exceptional charge storage capacity of MOFs, combined with their facile synthesis and scalability, makes them promising candidates for next-generation energy storage technologies. This review sheds light on the challenges and opportunities in the practical implementation of MOFs in energy storage devices and discusses strategies for enhancing the stability of MOFs in different environments, improving their electrical conductivity, and developing scalable synthesis methods. We briefly discuss perspectives and future directions, with particular focus on their research and development in the use of MOFs for energy storage applications.

金属有机框架的前沿:用于下一代超级电容器的创新纳米材料
金属有机框架(MOFs)是一类用途广泛的多孔材料,在包括储能设备在内的各种应用领域具有巨大潜力。本综述全面分析了 MOFs 在储能领域的最新进展和应用,包括对 MOFs 基本方面的简要概述,包括其合成、结构多样性和可调特性。人们对 MOFs 在超级电容器等先进储能系统中的应用进行了广泛的研究。MOFs 可用作电极材料、分离剂和催化剂,具有更强的电化学性能、更高的充放电速率和更长的循环稳定性。由于 MOFs 具有独特的可调性,因此可以合理地设计出具有所需特性的定制材料,如高比容量、优异的导电性和卓越的循环稳定性。基于 MOF 的电化学电容器的最新发展,尤其是在实现高能量和高功率密度方面取得的重大进展值得关注。MOFs 出色的电荷存储能力,加上其易于合成和可扩展性,使其成为下一代储能技术的理想候选材料。本综述揭示了在储能设备中实际应用 MOFs 所面临的挑战和机遇,并讨论了增强 MOFs 在不同环境中的稳定性、提高其导电性以及开发可扩展合成方法的策略。我们简要讨论了前景和未来的发展方向,尤其关注他们在将 MOFs 用于储能应用方面的研究和发展。
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来源期刊
CiteScore
26.00
自引率
21.40%
发文量
185
期刊介绍: Advanced Composites and Hybrid Materials is a leading international journal that promotes interdisciplinary collaboration among materials scientists, engineers, chemists, biologists, and physicists working on composites, including nanocomposites. Our aim is to facilitate rapid scientific communication in this field. The journal publishes high-quality research on various aspects of composite materials, including materials design, surface and interface science/engineering, manufacturing, structure control, property design, device fabrication, and other applications. We also welcome simulation and modeling studies that are relevant to composites. Additionally, papers focusing on the relationship between fillers and the matrix are of particular interest. Our scope includes polymer, metal, and ceramic matrices, with a special emphasis on reviews and meta-analyses related to materials selection. We cover a wide range of topics, including transport properties, strategies for controlling interfaces and composition distribution, bottom-up assembly of nanocomposites, highly porous and high-density composites, electronic structure design, materials synergisms, and thermoelectric materials. Advanced Composites and Hybrid Materials follows a rigorous single-blind peer-review process to ensure the quality and integrity of the published work.
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