Designing Moiré Patterns by Shearing

IF 16 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Pierre A. Pantaleón*, Héctor Sainz-Cruz and Francisco Guinea, 
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Abstract

We analyze the elastic properties, structural effects, and low-energy physics of a sheared nanoribbon placed on top of graphene, which creates a gradually changing moiré pattern. By means of a classical elastic model we derive the strains in the ribbon and we obtain its electronic energy spectrum with a scaled tight-binding model. The size of the sheared region is determined by the balance between elastic and van der Waals energy, and different regimes are identified. Near the clamped edge, moderate strains and small twist angles lead to one-dimensional channels. Near the sheared edge, a long region behaves like magic angle twisted bilayer graphene (TBG), showing a sharp peak in the density of states, mostly isolated from the rest of the spectrum. We also calculate the band topology along the ribbon and we find that it is stable for large intervals of strains and twist angles. Together with the experimental observations, these results show that the sheared nanoribbon geometry is ideal for exploring superconductivity and correlated phases in TBG in the very sought-after regime of ultralow twist angle disorder.

Abstract Image

通过剪切设计摩尔纹样
我们分析了放置在石墨烯顶部的剪切纳米带的弹性特性、结构效应和低能物理,它产生了逐渐变化的摩尔纹。通过经典弹性模型,我们推导出了纳米带中的应变,并通过缩放紧束模型获得了其电子能谱。剪切区域的大小由弹性能量和范德华能量之间的平衡决定,并确定了不同的状态。在夹紧边缘附近,适度的应变和较小的扭转角会产生一维通道。在剪切边缘附近,一个长区域表现得像魔角扭曲双层石墨烯(TBG),在状态密度中显示出一个尖锐的峰值,大部分与光谱的其余部分隔离。我们还计算了带状拓扑结构,发现它在较大的应变和扭曲角度范围内都很稳定。这些结果与实验观察结果一起表明,剪切纳米带的几何形状非常适合在超低扭转角无序状态下探索 TBG 的超导性和相关相。
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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