Suprovat Ghosh, Abir Mukherjee, Sudarshan Singh, Samit K Ray, Ananjan Basu, Santanu Manna and Samaresh Das*,
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引用次数: 0
Abstract
This article explores group-IV germanium (Ge) quantum dots (QDs) on silicon-on-insulator (SOI) grown by molecular beam epitaxy (MBE) in order to explore their optical behavior in the terahertz (THz) regime. In this work, Ge QDs, pumped by an above bandgap near–infrared wavelength, exhibit THz amplitude modulation in the frequency range of 0.1–1.0 THz. The epitaxial Ge QDs outperform the reference SOI (170 nm top Si) substrate in THz amplitude modulation due to higher carrier generation in weakly confined dots compared to their bulk counterpart. This is further corroborated using a theoretical model based on the nonequilibrium Green’s function (NEGF) method. This model enables the calculation of photocarrier generated (PCG) and their confinement in the Ge QD region. Our model also reroutes the calculation from PCG to the corresponding plasma frequency and hence to refractive index and THz photoconductivity. Moreover, the photogenerated confined holes’ accumulation at the Ge QDs/Si interface is elevated after optical illumination, leading to decreased THz photoconductivity. This augmentation in THz photoconductivity contributes to a significant enhancement of THz modulation depth of ∼77% at Ge QDs/Si interfaces compared to bare SOI at 0.1 THz.
期刊介绍:
ACS Applied Optical Materials is an international and interdisciplinary forum to publish original experimental and theoretical including simulation and modeling research in optical materials complementing the ACS Applied Materials portfolio. With a focus on innovative applications ACS Applied Optical Materials also complements and expands the scope of existing ACS publications that focus on fundamental aspects of the interaction between light and matter in materials science including ACS Photonics Macromolecules Journal of Physical Chemistry C ACS Nano and Nano Letters.The scope of ACS Applied Optical Materials includes high quality research of an applied nature that integrates knowledge in materials science chemistry physics optical science and engineering.