Combined contamination of tire and road wear microplastics with heavy metals in expressway tunnels: occurrence characteristics and risk assessment

IF 12.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Yanhua Wang, Na Xiao, Jian Zhao, Yu Su, Ziyi Guo, Bo Wang, Zhuanxi Luo, Hanzhong Jia, Baoshan Xing
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Abstract

Tire and road wear microplastics (TRWMPs), as an important type of microplastics, have attracted increasing attention. However, current studies on their contamination within expressway tunnels remain limited. Therefore, we investigated the occurrence characteristics of TRWMPs in dusts from various tunnels, and combined contamination with heavy metals (HMs). The results showed that the abundance of TRWMPs in expressway tunnel dust (53,778 n/kg) was much higher than that sampled from other land use types (1,360-4,960 n/kg) in the same region. A large amount of polyamide was released into the environment along with wear particles from the vehicles. Also, the abundance of TRWMPs inside tunnels was greater than outside, and the proportion of large-size TRWMPs was higher inside tunnels. TRWMPs was symmetrically distributed with respect to the center of expressway tunnel. The pollution load index (PLI) and ecological risk index (H) indicated that study area was heavily contaminated with TRWMPs. There was a significant positive correlation between the abundance of TRWMPs and concentration of Cr (p < 0.01) in dust, and their risk assessment and health risk fluctuations were almost identical. Thus, the study is of great significance for elucidating the synergistic contamination and potential risk of TRWMPs and HMs in expressway tunnels.

Abstract Image

高速公路隧道中轮胎和路面磨损微塑料与重金属的联合污染:发生特征与风险评估
轮胎和路面磨损微塑料(TRWMPs)作为一种重要的微塑料,已引起越来越多的关注。然而,目前对其在高速公路隧道内污染情况的研究仍然有限。因此,我们研究了不同隧道灰尘中 TRWMPs 的出现特征,并将其与重金属(HMs)污染结合起来。结果表明,高速公路隧道粉尘中 TRWMPs 的丰度(53,778 n/kg)远高于同一地区其他土地利用类型的粉尘样本(1,360-4,960 n/kg)。大量聚酰胺与车辆磨损颗粒一起释放到环境中。此外,隧道内 TRWMPs 的丰度高于隧道外,且隧道内大尺寸 TRWMPs 的比例较高。TRWMPs相对于高速公路隧道中心呈对称分布。污染负荷指数(PLI)和生态风险指数(H)表明,研究区域受到 TRWMPs 的严重污染。粉尘中 TRWMPs 的丰度与 Cr 的浓度(p < 0.01)之间存在明显的正相关,其风险评估和健康风险波动基本一致。因此,该研究对于阐明高速公路隧道中 TRWMPs 和 HMs 的协同污染和潜在风险具有重要意义。
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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