Effects of microplastics on the rheological properties of sediment slurries in aquatic environments

IF 10.3 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Jiaqi Zhang, Clarence Edward Choi, Feihong Gao
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Abstract

Sediment slurries, characterized by their high concentrations of fine-grained cohesive sediment, are prevalent in various aquatic environments, including fluid mud, sediment gravity flows, and dredging slurries. Abundant microplastics have been detected in sediment slurries, which indicates that these slurries function as carriers for the transport of microplastics. However, there is a dearth of understanding on how sediment slurries transport microplastics. To ascertain the transport mechanisms, elucidating the effects of microplastics on the rheological properties of sediment slurries is a prerequisite because these properties govern the flow dynamics and mobility of such slurries. This study conducts experimental and theoretical investigations to examine, interpret, and quantify the effects of microplastics on the rheological properties of sediment slurries. Microplastics are shown to increase the yield stress and viscosity of sediment slurries via enhancing sediment aggregation. A new descriptor, specifically, the effective volume fraction, is proposed to characterize the effects of microplastics on sediment aggregation. Based on the newly-proposed descriptor, a new analytical model is proposed to predict the yield stress and viscosity of sediment slurries with microplastics. This study lays a foundation for further interpretating the flow dynamics and thus the transport processes of sediment slurries laden with microplastics.
微塑料对水生环境中沉积泥浆流变特性的影响
沉积泥浆的特点是含有大量细粒粘性沉积物,普遍存在于各种水生环境中,包括流体泥浆、沉积物重力流和疏浚泥浆。在沉积泥浆中检测到了大量微塑料,这表明这些泥浆具有运输微塑料的载体功能。然而,人们对沉积泥浆如何迁移微塑料还缺乏了解。要确定其迁移机制,就必须阐明微塑料对沉积物泥浆流变特性的影响,因为这些特性会影响此类泥浆的流动动力学和流动性。本研究通过实验和理论研究来检查、解释和量化微塑料对沉积泥浆流变特性的影响。研究表明,微塑料可通过增强沉积物的聚集来提高沉积泥浆的屈服应力和粘度。为描述微塑料对沉积物聚集的影响,提出了一种新的描述指标,特别是有效体积分数。根据新提出的描述因子,提出了一个新的分析模型来预测含有微塑料的沉积泥浆的屈服应力和粘度。这项研究为进一步解释含有微塑料的沉积泥浆的流动动力学进而解释其迁移过程奠定了基础。
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来源期刊
Environment International
Environment International 环境科学-环境科学
CiteScore
21.90
自引率
3.40%
发文量
734
审稿时长
2.8 months
期刊介绍: Environmental Health publishes manuscripts focusing on critical aspects of environmental and occupational medicine, including studies in toxicology and epidemiology, to illuminate the human health implications of exposure to environmental hazards. The journal adopts an open-access model and practices open peer review. It caters to scientists and practitioners across all environmental science domains, directly or indirectly impacting human health and well-being. With a commitment to enhancing the prevention of environmentally-related health risks, Environmental Health serves as a public health journal for the community and scientists engaged in matters of public health significance concerning the environment.
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