Enhanced mass scattering efficiencies of background dust aerosols over East Asia following the passage of dust plumes

IF 4.2 2区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Chenguang Tang , Yingjing Lin , Pengfei Tian , Jinsen Shi , Tao Deng , Xuejiao Deng , Yu Zou , Lei Zhang
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Abstract

The transported dust particles significantly impact global weather and climate. Previous studies focused primarily on the physical and chemical properties of dust plumes, but the interaction mechanism between these dust plumes and background dust aerosols remains unclear. We explored this issue using in-situ observation data of the East Asia dust from the Semi-Arid Climate and Environment Observatory of Lanzhou University (SACOL) during January 2013. We identified a dust plume originating from the Gurbantunggut Desert, which triggered a four-day dust event with an average dust concentration of 67.2 μg m−3. Notably, this dust event led to a significant increase in mass scattering efficiencies of dust, shifting from an inverted U-shape to a continuously increasing pattern with wavelength. The enhanced dust mass scattering efficiency inhibited the development of the planetary boundary layer. These changes persisted for at least two weeks after the event, primarily due to the resuspension of deposited dust particles altering the size of background dust particle. Our findings highlight the ability of dust plumes to enhance the scattering efficiency of background dust aerosols and providing new insights into the complex interactions between dust and the atmosphere.
尘羽通过后东亚上空背景尘埃气溶胶的质量散射效率增强
飘移的尘埃粒子对全球天气和气候有重大影响。以往的研究主要关注沙尘卷的物理和化学性质,但这些沙尘卷与背景尘埃气溶胶之间的相互作用机制仍不清楚。我们利用兰州大学半干旱气候与环境观测站(SACOL)2013年1月对东亚沙尘的原位观测数据探讨了这一问题。我们确定了一股源自古尔班通古特沙漠的沙尘羽流,它引发了为期四天的沙尘事件,平均沙尘浓度为 67.2 μg m-3。值得注意的是,这次沙尘事件导致沙尘的质量散射效率显著增加,从倒 U 型转变为随波长持续增加的模式。尘埃质量散射效率的提高抑制了行星边界层的发展。这些变化在事件发生后至少持续了两周,主要是由于沉积尘粒的再悬浮改变了背景尘粒的大小。我们的研究结果凸显了尘羽提高背景尘埃气溶胶散射效率的能力,并为了解尘埃与大气之间复杂的相互作用提供了新的视角。
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来源期刊
Atmospheric Environment
Atmospheric Environment 环境科学-环境科学
CiteScore
9.40
自引率
8.00%
发文量
458
审稿时长
53 days
期刊介绍: Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.
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