CO2 valorisation from lime production via Columbus process to produce E-methane for transport sector – A comprehensive life cycle assessment

IF 7.2 2区 工程技术 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jordy Motte , Erasmo Cadena , Yblin Roman Escobar , Jim Gripekoven , Koen Vlaeminck , Friso De Clercq , Pierre-Olivier Cambier , Nathalie Van Den Bogaert , Brecht De Roo , Jan Mertens , Jo Dewulf
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Abstract

In the next decades, CO2 capture and utilisation (CCU) technologies can contribute to climate change mitigation. The Columbus project is an example of a CCU initiative in which CO2 is captured from lime production and converted into E-methane via CO2 methanation. E-methane can serve as fuel for ships and lorries to replace heavy fuel oil and diesel, respectively. This paper aims to assess the environmental impacts of E-methane production via the Columbus process, powered by renewable electricity, and its utilisation in the transport sector benchmarked to conventional fuel production (references) through life cycle assessment (LCA). A basket of products approach was used to also consider the co-products obtained from the Columbus process in the assessment. Both emission and resource based indicators were selected for the LCA. The results show that E-methane production and its utilisation in ships and lorries result in a decrease of the impact on climate change (35 %), particulate matter formation (94 %) and fossil resource use (85 %) compared to the references. For this comparison, the conventional production of the co-products was also taken into account. However, the production and utilisation of this fuel consumes more minerals and metals than the references. The higher mineral and metal extraction from the environment can be explained by the construction of the solar panels required to provide electricity for electrolysis. Future research should focus on the social acceptance and techno-economic assessment of the Columbus process.
通过哥伦布工艺将石灰生产过程中产生的二氧化碳变废为宝,为运输行业生产电子甲烷--综合生命周期评估
在未来几十年中,二氧化碳捕集与利用(CCU)技术将有助于减缓气候变化。哥伦布项目(Columbus project)就是二氧化碳捕集与利用(CCU)技术的一个实例,该项目从石灰生产中捕集二氧化碳,并通过二氧化碳甲烷化将其转化为电子甲烷(E-methane)。电子甲烷可作为船舶和卡车的燃料,分别替代重油和柴油。本文旨在通过生命周期评估(LCA),以可再生电力为动力,评估哥伦布工艺生产的甲烷对环境的影响,以及甲烷在运输行业的使用情况,并以传统燃料生产(参考)为基准进行评估。在评估中还采用了一篮子产品的方法,以考虑哥伦布工艺获得的副产品。生命周期评估选择了基于排放和资源的指标。结果表明,与参照物相比,电子甲烷的生产及其在船舶和卡车中的使用可减少对气候变化的影响(35%)、颗粒物的形成(94%)和化石资源的使用(85%)。在进行比较时,还考虑了副产品的常规生产。然而,这种燃料的生产和利用比参考值消耗更多的矿物和金属。从环境中提取更多矿物和金属的原因可能是建造了为电解提供电力所需的太阳能电池板。今后的研究应侧重于哥伦布工艺的社会接受度和技术经济评估。
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来源期刊
Journal of CO2 Utilization
Journal of CO2 Utilization CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.90
自引率
10.40%
发文量
406
审稿时长
2.8 months
期刊介绍: The Journal of CO2 Utilization offers a single, multi-disciplinary, scholarly platform for the exchange of novel research in the field of CO2 re-use for scientists and engineers in chemicals, fuels and materials. The emphasis is on the dissemination of leading-edge research from basic science to the development of new processes, technologies and applications. The Journal of CO2 Utilization publishes original peer-reviewed research papers, reviews, and short communications, including experimental and theoretical work, and analytical models and simulations.
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