Analysis of the National Air Pollutant Emissions Inventory (CAPSS 2018) Data and Assessment of Emissions Based on Air Quality Modeling in the Republic of Korea
Seong-woo Choi, Hyeonjeong Cho, Yumi Hong, Hee-ji Jo, Min Park, Hyeon-ji Lee, Ye-ji Choi, Ho-hyun Shin, Dongjae Lee, Eunji Shin, Wooseung Baek, Sung-kyu Park, Eunhye Kim, Hyung-cheon Kim, Seung-joo Song, Yunseo Park, Jinsik Kim, Jihye Baek, Jinsik Kim, Chul Yoo
{"title":"Analysis of the National Air Pollutant Emissions Inventory (CAPSS 2018) Data and Assessment of Emissions Based on Air Quality Modeling in the Republic of Korea","authors":"Seong-woo Choi, Hyeonjeong Cho, Yumi Hong, Hee-ji Jo, Min Park, Hyeon-ji Lee, Ye-ji Choi, Ho-hyun Shin, Dongjae Lee, Eunji Shin, Wooseung Baek, Sung-kyu Park, Eunhye Kim, Hyung-cheon Kim, Seung-joo Song, Yunseo Park, Jinsik Kim, Jihye Baek, Jinsik Kim, Chul Yoo","doi":"10.5572/ajae.2022.084","DOIUrl":null,"url":null,"abstract":"<div><p>According to the 2018 National Air Pollutant Emissions Inventory (NEI), air pollutant emissions in the Republic of Korea comprised 808,801 tons of CO, 1,153,265 tons of NO<sub>X</sub>, 300,979 tons of SO<sub>X</sub>, 617,481 tons of TSP, 232,993 tons of PM<sub>10</sub>, 98,388 tons of PM<sub>2.5</sub>, 15,562 tons of black carbon (BC), 1,035,636 tons of VOCs, and 315,975 tons of NH<sub>3</sub>. As for national emission contributions to primary PM<sub>2.5</sub> and PM precursors (NO<sub>X</sub>, SO<sub>X</sub>, VOCs, and NH<sub>3</sub>), major source categories were the road sector for NO<sub>X</sub>, the industry sector for SO<sub>X</sub> and PM<sub>2.5</sub>, and the everyday activities and others sector for VOCs and NH<sub>3</sub>. In the case of emissions by region, the largest amount of NO<sub>X</sub> was emitted from the Seoul Metropolitan Areas (SMA; Seoul, Incheon, and Gyeonggi-do, hereafter SMA) and the largest amounts of SO<sub>X</sub>, PM<sub>2.5</sub>, VOCs, and NH<sub>3</sub> were from the Yeongnam region. A 3D chemical transport modeling system was used to examine the uncertainty of the national air pollutant emissions based on the National Emission and Air Quality Assessment System (NEAS). Air quality was simulated using CAPSS 2018, and the simulation data were compared with observed concentrations to examine the uncertainties of the current emissions. These data show that emissions from five si (cities) (Pohang, Yeosu, Gwangyang, Dangjin, and Ulsan) need to be improved. Most of all, it is necessary to examine the emissions from places of business that use anthracite, which is the major PM<sub>2.5</sub> emission source, as fuel in these areas.</p></div>","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2022-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.5572/ajae.2022.084.pdf","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"1085","ListUrlMain":"https://link.springer.com/article/10.5572/ajae.2022.084","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
According to the 2018 National Air Pollutant Emissions Inventory (NEI), air pollutant emissions in the Republic of Korea comprised 808,801 tons of CO, 1,153,265 tons of NOX, 300,979 tons of SOX, 617,481 tons of TSP, 232,993 tons of PM10, 98,388 tons of PM2.5, 15,562 tons of black carbon (BC), 1,035,636 tons of VOCs, and 315,975 tons of NH3. As for national emission contributions to primary PM2.5 and PM precursors (NOX, SOX, VOCs, and NH3), major source categories were the road sector for NOX, the industry sector for SOX and PM2.5, and the everyday activities and others sector for VOCs and NH3. In the case of emissions by region, the largest amount of NOX was emitted from the Seoul Metropolitan Areas (SMA; Seoul, Incheon, and Gyeonggi-do, hereafter SMA) and the largest amounts of SOX, PM2.5, VOCs, and NH3 were from the Yeongnam region. A 3D chemical transport modeling system was used to examine the uncertainty of the national air pollutant emissions based on the National Emission and Air Quality Assessment System (NEAS). Air quality was simulated using CAPSS 2018, and the simulation data were compared with observed concentrations to examine the uncertainties of the current emissions. These data show that emissions from five si (cities) (Pohang, Yeosu, Gwangyang, Dangjin, and Ulsan) need to be improved. Most of all, it is necessary to examine the emissions from places of business that use anthracite, which is the major PM2.5 emission source, as fuel in these areas.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.