Nitrogen Trifluoride Emissions in China from 2017 to 2021 Derived from Atmospheric Observations

IF 8.9 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Wenbin Weng, Minde An, Luke M. Western, Ronald G. Prinn, Jianxin Hu, Xingchen Zhao, Matthew Rigby, Yinuo Wang, Siyuan Huang, Honghui Xu, Yan Yu, Wenxue Chi and Bo Yao*, 
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Abstract

Rapid growth in the emissions of nitrogen trifluoride (NF3), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF3 emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF3 emissions in China increased from 0.95 (0.82–1.07) Gg yr–1 in 2017 to 1.41 (1.28–1.55) Gg yr–1 in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF3 emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr–1is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr–1) over the same period. We identified substantial NF3 emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF3 emissions. Moreover, large NF3 emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF3 emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.

根据大气观测数据推算的 2017-2021 年中国三氟化氮排放量
三氟化氮(NF3)是一种强效温室气体,其排放量的快速增长对环境和气候系统构成了威胁。本研究基于中国9个背景站的大气观测数据,采用基于拉格朗日-色散模型的贝叶斯反演技术,估算了2017年至2021年中国的三氟化氮排放量及其空间分布。我们发现,中国的 NF3 排放量从 2017 年的 0.95(0.82-1.07)Gg yr-1 增加到 2021 年的 1.41(1.28-1.55)Gg yr-1,在此期间大幅增长了 48%。2017-2020 年间,中国 NF3 排放量的绝对增幅为 0.65 (0.57-0.74) 千兆克/年-1,与同期全球排放量的增幅(0.63 (0.50-0.75) 千兆克/年-1)相当。我们在珠江三角洲和长江三角洲地区以及湖北省发现了大量的三氟化氮排放,这些地区完善的半导体工业可能是三氟化氮排放的来源。此外,在华北地区,包括河北省、河南省和山东省,也发现了大量的 NF3 排放。如果不采取控制措施,NF3排放量的增加可能会推迟中国到 2060 年实现碳中和目标的进程。
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来源期刊
Environmental Science & Technology Letters Environ.
Environmental Science & Technology Letters Environ. ENGINEERING, ENVIRONMENTALENVIRONMENTAL SC-ENVIRONMENTAL SCIENCES
CiteScore
17.90
自引率
3.70%
发文量
163
期刊介绍: Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.
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