Solar-Driven Evaporator With "Starburst Turbine" Design Featuring Directional Salt Crystallization, Antibacterial, and Catalytic Multifunctionality for Efficient Water Purification.

IF 14.3 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jiahui Yu, Lele Li, Yuxuan Liu, Jie Wen, Shu Liu, Jiye Li, Junyi Ning, Changxiang Shao, Tao Wu, Bing Liu
{"title":"Solar-Driven Evaporator With \"Starburst Turbine\" Design Featuring Directional Salt Crystallization, Antibacterial, and Catalytic Multifunctionality for Efficient Water Purification.","authors":"Jiahui Yu, Lele Li, Yuxuan Liu, Jie Wen, Shu Liu, Jiye Li, Junyi Ning, Changxiang Shao, Tao Wu, Bing Liu","doi":"10.1002/advs.202406696","DOIUrl":null,"url":null,"abstract":"<p><p>Facing the global challenge of water scarcity, solar-driven desalination is considered a sustainable technology for obtaining freshwater from seawater. However, issues such as uncontrolled salt crystallization and bacterial contamination limit its efficiency and practicality. This study proposes an innovative solar-driven evaporator designed to address these challenges using optimized shape design and advanced photothermal materials. Based on finite element analyses, cylindrical evaporators with a \"Starburst Turbine\" shape are designed and fabricated, achieving directional salt crystallization and a record-breaking water collection rate of 3.56 kg m<sup>-2</sup> h<sup>-1</sup> and an evaporation rate of 4.57 kg m<sup>-2</sup> h<sup>-1</sup> under one sun illumination. During continuous 60-h illumination tests, the evaporator maintained a stable evaporation rate, attributed to its excellent directional salt crystallization capability. Additionally, the evaporator demonstrates superior photodynamic antibacterial performance and photocatalytic degradation of organic pollutants. Under one sun illumination for 1 h, it achieves 100% sterilization of S. aureus and E. coli, and a 95.4% degradation of methylene blue (MB), demonstrating its potential to purify various wastewater types. These findings underscore the significant scientific and practical value of integrating antibacterial and photocatalytic functions into solar water purification materials, providing a sustainable solution to global water scarcity challenges and environmental protection.</p>","PeriodicalId":117,"journal":{"name":"Advanced Science","volume":null,"pages":null},"PeriodicalIF":14.3000,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Science","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/advs.202406696","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Facing the global challenge of water scarcity, solar-driven desalination is considered a sustainable technology for obtaining freshwater from seawater. However, issues such as uncontrolled salt crystallization and bacterial contamination limit its efficiency and practicality. This study proposes an innovative solar-driven evaporator designed to address these challenges using optimized shape design and advanced photothermal materials. Based on finite element analyses, cylindrical evaporators with a "Starburst Turbine" shape are designed and fabricated, achieving directional salt crystallization and a record-breaking water collection rate of 3.56 kg m-2 h-1 and an evaporation rate of 4.57 kg m-2 h-1 under one sun illumination. During continuous 60-h illumination tests, the evaporator maintained a stable evaporation rate, attributed to its excellent directional salt crystallization capability. Additionally, the evaporator demonstrates superior photodynamic antibacterial performance and photocatalytic degradation of organic pollutants. Under one sun illumination for 1 h, it achieves 100% sterilization of S. aureus and E. coli, and a 95.4% degradation of methylene blue (MB), demonstrating its potential to purify various wastewater types. These findings underscore the significant scientific and practical value of integrating antibacterial and photocatalytic functions into solar water purification materials, providing a sustainable solution to global water scarcity challenges and environmental protection.

采用 "星爆涡轮 "设计的太阳能驱动蒸发器,具有定向盐结晶、抗菌和催化多功能性,可实现高效水净化。
面对全球缺水的挑战,太阳能驱动的海水淡化技术被认为是从海水中获取淡水的可持续技术。然而,盐结晶失控和细菌污染等问题限制了其效率和实用性。本研究提出了一种创新的太阳能驱动蒸发器,旨在利用优化的形状设计和先进的光热材料来应对这些挑战。在有限元分析的基础上,设计并制造了具有 "星爆涡轮 "形状的圆柱形蒸发器,实现了盐的定向结晶,并在一个太阳光照下实现了破纪录的 3.56 kg m-2 h-1 的水收集率和 4.57 kg m-2 h-1 的蒸发率。在连续 60 小时的光照测试中,蒸发器保持了稳定的蒸发率,这归功于其出色的定向盐结晶能力。此外,该蒸发器还具有卓越的光动力抗菌性能和光催化降解有机污染物的能力。在太阳光照射 1 小时的情况下,金黄色葡萄球菌和大肠杆菌的杀菌率达到 100%,亚甲基蓝(MB)的降解率达到 95.4%,显示了其净化各类废水的潜力。这些发现强调了将抗菌和光催化功能集成到太阳能净水材料中的重要科学和实用价值,为应对全球水资源短缺挑战和环境保护提供了可持续的解决方案。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Advanced Science
Advanced Science CHEMISTRY, MULTIDISCIPLINARYNANOSCIENCE &-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
18.90
自引率
2.60%
发文量
1602
审稿时长
1.9 months
期刊介绍: Advanced Science is a prestigious open access journal that focuses on interdisciplinary research in materials science, physics, chemistry, medical and life sciences, and engineering. The journal aims to promote cutting-edge research by employing a rigorous and impartial review process. It is committed to presenting research articles with the highest quality production standards, ensuring maximum accessibility of top scientific findings. With its vibrant and innovative publication platform, Advanced Science seeks to revolutionize the dissemination and organization of scientific knowledge.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信