{"title":"Local-field corrections of the Green's tensor in chiral media","authors":"Janine C. Franz, Stefan Yoshi Buhmann, A. Salam","doi":"10.1103/physreva.110.033109","DOIUrl":null,"url":null,"abstract":"In this paper we derive local-field corrections for interactions within chiral media using the Onsager real cavity model. The problem is not fully solvable analytically, so we introduce a matrix formalism to determine the correct local-field corrections. We find that left- and right-handed circularly polarized excitations yield different correction factors inside a chiral medium, analogous to their different propagation velocities. These chiral correction factors can significantly alter theoretical predictions for chiral effects within the medium. We validate our solution in various limits and special cases, particularly when the source and absorption points coincide, enabling analytical comparison for nonabsorbing media. For spontaneous emission in a chiral medium, we extend the local-field correction to absorbing media, revealing fundamentally different corrections analogous to the nonchiral case.","PeriodicalId":20146,"journal":{"name":"Physical Review A","volume":"4 1","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2024-09-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review A","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physreva.110.033109","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"Physics and Astronomy","Score":null,"Total":0}
引用次数: 0
Abstract
In this paper we derive local-field corrections for interactions within chiral media using the Onsager real cavity model. The problem is not fully solvable analytically, so we introduce a matrix formalism to determine the correct local-field corrections. We find that left- and right-handed circularly polarized excitations yield different correction factors inside a chiral medium, analogous to their different propagation velocities. These chiral correction factors can significantly alter theoretical predictions for chiral effects within the medium. We validate our solution in various limits and special cases, particularly when the source and absorption points coincide, enabling analytical comparison for nonabsorbing media. For spontaneous emission in a chiral medium, we extend the local-field correction to absorbing media, revealing fundamentally different corrections analogous to the nonchiral case.
期刊介绍:
Physical Review A (PRA) publishes important developments in the rapidly evolving areas of atomic, molecular, and optical (AMO) physics, quantum information, and related fundamental concepts.
PRA covers atomic, molecular, and optical physics, foundations of quantum mechanics, and quantum information, including:
-Fundamental concepts
-Quantum information
-Atomic and molecular structure and dynamics; high-precision measurement
-Atomic and molecular collisions and interactions
-Atomic and molecular processes in external fields, including interactions with strong fields and short pulses
-Matter waves and collective properties of cold atoms and molecules
-Quantum optics, physics of lasers, nonlinear optics, and classical optics