Matthew Phillips, Muh-Jang Chen, Jong Ryu, Mohammed Zikry
{"title":"Dynamic Behavior of Ribbed Viscoelastic CNT-PDMS Thin-Films for Multifunctional Applications","authors":"Matthew Phillips, Muh-Jang Chen, Jong Ryu, Mohammed Zikry","doi":"10.1002/mame.202400098","DOIUrl":null,"url":null,"abstract":"<p>Tailored ribbing structures are obtained by large-scale rolling in polymer PDMS thin-films by adding carbon nanotubes (CNT) inclusions, which significantly improved the mechanical behavior of systems subjected to dynamic compressive strain rates. A nonlinear explicit dynamic three-dimensional finite-element (FE) scheme is used to understand and predict the thermomechanical response of the manufactured ribbed thin-film structures subjected to dynamic in-plane compressive loading. Representative volume element (RVE) FE models of the ribbed thin-films are subjected to strain rates as high as 10<sup>4</sup> s<sup>−1</sup> in both the transverse and parallel ribbing directions. Latin Hypercube Sampling of the microstructural parameters, as informed from experimental observations, provide the microstructurally based RVEs. An interior-point optimization routine is also employed on a regression model trained from the FE predictions that can be used to design ribbed materials for multifunctional applications. The model verifies that damage can be mitigated in CNT-PDMS systems subjected to dynamic compressive loading conditions by controlling the ribbing microstructural characteristics, such as the film thickness and the ribbing amplitude and wavelength. This approach provides a framework for designing materials that can be utilized for applications that require high strain rate damage tolerance, drag reduction, antifouling, and superhydrophobicity.</p>","PeriodicalId":18151,"journal":{"name":"Macromolecular Materials and Engineering","volume":null,"pages":null},"PeriodicalIF":4.2000,"publicationDate":"2024-09-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/mame.202400098","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Macromolecular Materials and Engineering","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/mame.202400098","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Tailored ribbing structures are obtained by large-scale rolling in polymer PDMS thin-films by adding carbon nanotubes (CNT) inclusions, which significantly improved the mechanical behavior of systems subjected to dynamic compressive strain rates. A nonlinear explicit dynamic three-dimensional finite-element (FE) scheme is used to understand and predict the thermomechanical response of the manufactured ribbed thin-film structures subjected to dynamic in-plane compressive loading. Representative volume element (RVE) FE models of the ribbed thin-films are subjected to strain rates as high as 104 s−1 in both the transverse and parallel ribbing directions. Latin Hypercube Sampling of the microstructural parameters, as informed from experimental observations, provide the microstructurally based RVEs. An interior-point optimization routine is also employed on a regression model trained from the FE predictions that can be used to design ribbed materials for multifunctional applications. The model verifies that damage can be mitigated in CNT-PDMS systems subjected to dynamic compressive loading conditions by controlling the ribbing microstructural characteristics, such as the film thickness and the ribbing amplitude and wavelength. This approach provides a framework for designing materials that can be utilized for applications that require high strain rate damage tolerance, drag reduction, antifouling, and superhydrophobicity.
期刊介绍:
Macromolecular Materials and Engineering is the high-quality polymer science journal dedicated to the design, modification, characterization, and processing of advanced polymeric materials.