Enhancing the Efficiency of Ultra-thin Perovskite Solar Cell Through Cluster of Cubic Plasmonic Nanoparticles: A Numerical Investigation

IF 3.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL
Amir Hossein Mohammadian Fard, Samiye Matloub
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Abstract

Perovskite solar cells have emerged as a promising third-generation solar cell technology, characterized by high efficiency and low fabrication costs, garnering significant research attention in recent years. In this study, the impact of embedding the cluster of cubic plasmonic nanoparticles within the ultra-thin absorber layer of perovskite solar cells was investigated. Various types of metallic nanoparticles (including Au, Ag, Al, and Cu) were employed in the perovskite absorber layer, each with different thicknesses and widths. This facilitated a comprehensive comparison aimed at identifying the optimal structure for light absorption within the bandgap range of the perovskite absorber layer—specifically, 300 to 800 nm, corresponding to a bandgap energy of 1.55 eV. The layers used in the design of the perovskite solar cell in this research are SiO2/ITO/SnO2/MAPbI3/MoO3/Au. Optical and electrical analyses revealed that the local field intensity is significantly stronger at the edges of metallic nanoparticles. Notably, the efficiency of perovskite solar cells is enhanced by 56.87% (rising from 18.24 to 28.62%) with the incorporation of an Ag-based cluster of cubic nanoparticles, compared to perovskite solar cells without metallic nanoparticles. This achievement resulted in an overall efficiency of 28.62% and a short-circuit current of 31.22 mA/cm2. This result closely approaches the efficiency limitation of perovskite absorber layers, which indicates the potential for significant performance enhancements in future perovskite solar cell technologies.

Abstract Image

通过立方质子纳米粒子簇提高超薄过氧化物太阳能电池的效率:数值研究
透镜太阳能电池是一种前景广阔的第三代太阳能电池技术,具有效率高、制造成本低的特点,近年来备受研究关注。本研究探讨了在过氧化物太阳能电池的超薄吸收层中嵌入立方质子纳米粒子簇的影响。在包晶石吸收层中采用了各种类型的金属纳米粒子(包括金、银、铝和铜),每种粒子的厚度和宽度各不相同。这有助于进行全面比较,以确定在透辉石吸收层带隙范围内(即 300 至 800 纳米,相当于 1.55 eV 带隙能)的最佳光吸收结构。本研究设计的透辉石太阳能电池使用的层为 SiO2/ITO/SnO2/MAPbI3/MoO3/Au。光学和电学分析表明,金属纳米粒子边缘的局部场强明显更强。值得注意的是,与不含金属纳米颗粒的透辉石太阳能电池相比,加入银基立方纳米颗粒簇后,透辉石太阳能电池的效率提高了 56.87%(从 18.24% 提高到 28.62%)。这一成果的总体效率为 28.62%,短路电流为 31.22 mA/cm2。这一结果接近于包晶石吸收层的效率极限,这表明未来的包晶石太阳能电池技术具有显著提高性能的潜力。
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来源期刊
Plasmonics
Plasmonics 工程技术-材料科学:综合
CiteScore
5.90
自引率
6.70%
发文量
164
审稿时长
2.1 months
期刊介绍: Plasmonics is an international forum for the publication of peer-reviewed leading-edge original articles that both advance and report our knowledge base and practice of the interactions of free-metal electrons, Plasmons. Topics covered include notable advances in the theory, Physics, and applications of surface plasmons in metals, to the rapidly emerging areas of nanotechnology, biophotonics, sensing, biochemistry and medicine. Topics, including the theory, synthesis and optical properties of noble metal nanostructures, patterned surfaces or materials, continuous or grated surfaces, devices, or wires for their multifarious applications are particularly welcome. Typical applications might include but are not limited to, surface enhanced spectroscopic properties, such as Raman scattering or fluorescence, as well developments in techniques such as surface plasmon resonance and near-field scanning optical microscopy.
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