Wettability gradient of photoresponsive electrospun yarns for harp-based fog water harvesting

IF 7.9 2区 综合性期刊 Q1 CHEMISTRY, MULTIDISCIPLINARY
Gregory Parisi, Piotr K. Szewczyk, Shankar Narayan, Urszula Stachewicz
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Abstract

Fog water harvesting offers a solution to water scarcity. Here, we introduce a method to enhance fog water harvesting systems utilizing electrospun yarns featuring a wettability gradient. These yarns, made from polyvinylidene fluoride (PVDF) and titanium dioxide (TiO2), gain photoinduced hydrophilicity under UV light due to TiO2 photocatalytic properties, allowing dynamic shifts from hydrophobic to hydrophilic states. Experiments show that an alternating PVDF-TiO2 harp with a wettability gradient surpasses purely hydrophobic or hydrophilic versions in fog collection. The strategic mix of hydrophobic and hydrophilic sections enhances droplet movement and water capture, achieving a 16% increase in collection rate up to 400 mg cm−2 h−1. This approach introduces a novel method for creating wettability gradients in electrospun yarns via UV irradiation and represents a significant advancement in adaptable fog water harvesting systems.

Abstract Image

用于竖琴式雾水收集的光致伸缩电纺纱的润湿梯度
雾水收集为水资源短缺提供了一种解决方案。在此,我们介绍一种利用具有润湿梯度的电纺纱来增强雾水收集系统的方法。这些纱线由聚偏二氟乙烯(PVDF)和二氧化钛(TiO2)制成,由于二氧化钛的光催化特性,这些纱线在紫外线照射下可获得光诱导亲水性,从而实现从疏水状态到亲水状态的动态转变。实验表明,具有润湿梯度的 PVDF-TiO2 交替竖琴在雾气收集方面优于纯疏水性或亲水性竖琴。疏水和亲水部分的策略性混合增强了水滴的移动和水捕获,使收集率提高了 16%,最高可达 400 毫克厘米-2 小时-1。这种方法介绍了一种通过紫外线照射在电纺纱中产生润湿性梯度的新方法,是适应性雾水收集系统的一大进步。
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来源期刊
Cell Reports Physical Science
Cell Reports Physical Science Energy-Energy (all)
CiteScore
11.40
自引率
2.20%
发文量
388
审稿时长
62 days
期刊介绍: Cell Reports Physical Science, a premium open-access journal from Cell Press, features high-quality, cutting-edge research spanning the physical sciences. It serves as an open forum fostering collaboration among physical scientists while championing open science principles. Published works must signify significant advancements in fundamental insight or technological applications within fields such as chemistry, physics, materials science, energy science, engineering, and related interdisciplinary studies. In addition to longer articles, the journal considers impactful short-form reports and short reviews covering recent literature in emerging fields. Continually adapting to the evolving open science landscape, the journal reviews its policies to align with community consensus and best practices.
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