Qingson Jing, Ming Zhou, Baoying Lu, Xiao Li, Jianxin Wang, Naiyao Mao
{"title":"Lubrication Performance Under Electrical Regulation: Investigating the Mechanism of Graphene/Ionic Liquid Composite Materials","authors":"Qingson Jing, Ming Zhou, Baoying Lu, Xiao Li, Jianxin Wang, Naiyao Mao","doi":"10.1007/s11249-024-01907-8","DOIUrl":null,"url":null,"abstract":"<div><p>To delve into the mechanisms of lubricating additives in electrically charged environments, this study utilizes a non-covalent modification method combining N-butylpyridinium tetrafluoroborate ([BPy]BF<sub>4</sub>) with multilayer graphene (MG) to create graphene/ionic liquid (G/IL) composites. These composites were tested as lubricating additives in polyalphaolefin 40 (PAO40) using the UMT-2 experimental platform to assess their performance and electrical regulation mechanisms. Results demonstrated that G/IL composites significantly enhance lubrication and electrical stability. The study discovered that varying the current’s intensity and polarity substantially influences ion concentration and Zeta potential at the interface, reducing the electroviscous effect and facilitating the formation of an interfacial adsorption film. The interplay of these mechanisms greatly optimizes the interface condition. Additionally, real-time contact resistance data indicated a correlation between friction coefficient and contact resistance, validating the synergistic effect’s impact. This research not only clarifies the complex action mechanisms of lubricating additives in charged conditions but also offers critical insights for designing highly efficient lubricating materials.</p></div>","PeriodicalId":806,"journal":{"name":"Tribology Letters","volume":"72 4","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2024-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Tribology Letters","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s11249-024-01907-8","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
To delve into the mechanisms of lubricating additives in electrically charged environments, this study utilizes a non-covalent modification method combining N-butylpyridinium tetrafluoroborate ([BPy]BF4) with multilayer graphene (MG) to create graphene/ionic liquid (G/IL) composites. These composites were tested as lubricating additives in polyalphaolefin 40 (PAO40) using the UMT-2 experimental platform to assess their performance and electrical regulation mechanisms. Results demonstrated that G/IL composites significantly enhance lubrication and electrical stability. The study discovered that varying the current’s intensity and polarity substantially influences ion concentration and Zeta potential at the interface, reducing the electroviscous effect and facilitating the formation of an interfacial adsorption film. The interplay of these mechanisms greatly optimizes the interface condition. Additionally, real-time contact resistance data indicated a correlation between friction coefficient and contact resistance, validating the synergistic effect’s impact. This research not only clarifies the complex action mechanisms of lubricating additives in charged conditions but also offers critical insights for designing highly efficient lubricating materials.
期刊介绍:
Tribology Letters is devoted to the development of the science of tribology and its applications, particularly focusing on publishing high-quality papers at the forefront of tribological science and that address the fundamentals of friction, lubrication, wear, or adhesion. The journal facilitates communication and exchange of seminal ideas among thousands of practitioners who are engaged worldwide in the pursuit of tribology-based science and technology.