Fabrication of graphene-plant fiber hybrid aerogel and its application for treatment of tritiated pump oil

IF 1.5 3区 化学 Q3 CHEMISTRY, ANALYTICAL
Shi Chen, Yu-Jia Xiao, Yan-Rong He
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Abstract

Due to the rapid development of fusion energy, the treatment of tritium-containing organic waste liquid has attracted significant attention. In this work, with plant fiber as an additive, the grpahene-plant fiber hybrid aerogel (G/P-A) was fabricated and used to adsorb tritiated pump oil. Results show that, compared to pure graphene aerogel (G-A), G/P-A displays better equal volume adsorption capacity (Qv) and higher adsorption efficiency. For pump oil, the maximum adsorption capacity was 49.39 mg/mg, and Qv reached an impressive 663.2 mg/mL, which is 17.82% higher than G-A (562.9 mg/mL). For other different adsorption targets, the maximum adsorption capacity ranged from 38.9 to 52.1 mg/mg is obtained. Due to its cost-effectiveness, strong oil absorption capability, and resistance to radiation, G/P-A could be a promising candidate for the adsorption treatment of tritium-containing organic waste liquid, such as tritiated pump oil.

Graphical abstract

Abstract Image

石墨烯-植物纤维混合气凝胶的制备及其在三硝化泵油处理中的应用
随着核聚变能源的飞速发展,含氚有机废液的处理备受关注。本研究以植物纤维为添加剂,制备了石墨烯-植物纤维混合气凝胶(G/P-A),并将其用于吸附氚泵油。结果表明,与纯石墨烯气凝胶(G-A)相比,G/P-A 具有更好的等体积吸附容量(Qv)和更高的吸附效率。对于泵油,最大吸附容量为 49.39 毫克/毫克,Qv 达到惊人的 663.2 毫克/毫升,比 G-A(562.9 毫克/毫升)高出 17.82%。对于其他不同的吸附目标,最大吸附容量介于 38.9 至 52.1 毫克/毫克之间。由于其成本效益高、吸油能力强且耐辐射,G/P-A 有望成为吸附处理含氚有机废液(如氚泵油)的候选材料。
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来源期刊
CiteScore
2.80
自引率
18.80%
发文量
504
审稿时长
2.2 months
期刊介绍: An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.
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