Anode-free post-Li metal batteries

IF 12.2 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Deik Petersen, Monja Gronenberg, German Lener, Ezequiel P. M. Leiva, Guillermina L. Luque, Sasan Rostami, Andrea Paolella, Bing Joe Hwang, Rainer Adelung and Mozaffar Abdollahifar
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Abstract

Anode-free metal batteries (AFMBs) are a new architecture of battery technology that relies solely on current collectors (CCs) at the anode side, eliminating the need for traditional metal anodes. This approach can pave the way for higher energy densities, lower manufacturing costs, and lower environmental footprints associated with metal batteries. This comprehensive review provides an in-depth exploration of AFMB technology, extending its scope beyond lithium and into a broader range of metals (sodium Na, potassium K, magnesium Mg, zinc Zn and aluminum Al). The concept of “metal-philicity” is discussed, which plays a pivotal role in understanding and controlling metal plating behavior within AFMBs, and also computational studies that employ first-principles calculations. This novel notion offers valuable insights into the interactions between metals and CC surfaces, which are essential for designing efficient battery systems. Moreover, the review explores various materials and experimental methods to enhance metal plating efficiency while mitigating issues such as dendrite formation through the realm of surface modifications and coatings on CCs. By providing a deeper understanding of strategies for optimizing anode-free post-Li metal battery technologies, this review aims to contribute to developing more efficient, sustainable, and cost-effective energy storage for the near future.

Abstract Image

Abstract Image

无阳极后锂金属电池
无阳极金属电池(AFMB)是一种新的电池技术结构,它完全依靠阳极侧的电流收集器(CC),无需传统的金属阳极。这种方法可以为提高能量密度、降低制造成本以及减少与金属电池相关的环境足迹铺平道路。本综述深入探讨了 AFMB 技术,将其范围从锂扩展到更广泛的金属(钠 Na、钾 K、镁 Mg、锌 Zn 和铝 Al)。文中讨论了 "金属亲和性 "的概念,这一概念在理解和控制 AFMB 中的金属电镀行为以及采用第一原理计算的计算研究中发挥着关键作用。这一新颖的概念为了解金属与 CC 表面之间的相互作用提供了宝贵的见解,这对于设计高效的电池系统至关重要。此外,该综述还探讨了各种材料和实验方法,以提高金属电镀效率,同时通过对 CC 进行表面改性和涂层来缓解枝晶形成等问题。通过深入了解优化无阳极后锂金属电池技术的策略,本综述旨在为不久的将来开发更高效、更可持续、更具成本效益的储能技术做出贡献。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Materials Horizons
Materials Horizons CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
18.90
自引率
2.30%
发文量
306
审稿时长
1.3 months
期刊介绍: Materials Horizons is a leading journal in materials science that focuses on publishing exceptionally high-quality and innovative research. The journal prioritizes original research that introduces new concepts or ways of thinking, rather than solely reporting technological advancements. However, groundbreaking articles featuring record-breaking material performance may also be published. To be considered for publication, the work must be of significant interest to our community-spanning readership. Starting from 2021, all articles published in Materials Horizons will be indexed in MEDLINE©. The journal publishes various types of articles, including Communications, Reviews, Opinion pieces, Focus articles, and Comments. It serves as a core journal for researchers from academia, government, and industry across all areas of materials research. Materials Horizons is a Transformative Journal and compliant with Plan S. It has an impact factor of 13.3 and is indexed in MEDLINE.
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