Quantum Conductivity in Single and Coupled Quantum-Dimensional Particles of Narrow-Gap Semiconductors

IF 0.6 4区 物理与天体物理 Q4 PHYSICS, CONDENSED MATTER
M. V. Gavrikov, E. G. Glukhovskoy, N. D. Zhukov
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Abstract

An organo-modified ordered layered structure with three-dimensional close packing based on colloidal quantumsized particles (QP) of InSb, PbS, CdSe semiconductors and Langmuir–Blodgett films has been fabricated and studied. According to the current-voltage characteristics (CVC) of single-electron transport in the model of a nanocell with a linear chain QP across the layers, the processes limiting conductivity were established: emission–injection tunneling from a probe into a nanoparticle, motion in a nanoparticle determined by the establishment of an electronic wave process in it, and tunneling through a nanogap between nanoparticles. Quasi-periodic oscillations of the current and resonant peaks of quantum conductivity are observed on the I–V characteristics, which were estimated in the quantum wire model. For an even number of layers (QP, 2, or 4), the I–V characteristics were used to determine the attenuation of size quantization and the decrease in current due to the weak interaction of nanoparticles. With an odd number (3 or 5), the nanochain acts as a single quantum thread with manifestations on the CVC similar to the cases of one QP. In this case, the motion of an electron can be considered as a one-electron charge wave.

Abstract Image

窄隙半导体单个和耦合量子维粒子的量子传导性
摘要 以 InSb、PbS、CdSe 半导体的胶体量子化颗粒(QP)和 Langmuir-Blodgett 薄膜为基础,制备并研究了具有三维紧密堆积的有机修饰有序层状结构。根据具有跨层线性链 QP 的纳米电池模型中单电子传输的电流-电压特性 (CVC),确定了限制导电性的过程:从探针到纳米粒子的发射-注入隧穿、由纳米粒子中电子波过程的建立决定的纳米粒子中的运动以及通过纳米粒子之间的纳米间隙的隧穿。根据量子线模型的估算,在 I-V 特性上可以观察到电流的准周期振荡和量子电导率的共振峰。对于偶数层(QP、2 或 4),I-V 特性用于确定尺寸量子化的衰减和纳米粒子弱相互作用导致的电流下降。当数量为奇数(3 或 5)时,纳米链就像一条量子线,在 CVC 上的表现与一个 QP 的情况类似。在这种情况下,电子的运动可视为单电子电荷波。
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来源期刊
Semiconductors
Semiconductors 物理-物理:凝聚态物理
CiteScore
1.50
自引率
28.60%
发文量
131
审稿时长
3-6 weeks
期刊介绍: Publishes the most important work in semiconductor research in the countries of the former Soviet Union. Covers semiconductor theory, transport phenomena in semiconductors, optics, magnetooptics, and electrooptics of semiconductors, semiconductor lasers and semiconductor surface physics. The journal features an extensive book review section.
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