Emerging collective quantum phenomena of excitons in metal-halide perovskites

IF 4.1 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Ajay K. Poonia, Parashurama Salunkhe, Angshuman Nag, K. V. Adarsh
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引用次数: 0

Abstract

Metal-halide perovskites (MHPs) with unique electronic and optical properties have emerged as promising materials with a broad spectrum of applications in photovoltaics, optoelectronic, and photonic devices. The distinct properties and tremendous potential of MHPs are intricately defined by excitons and collective quantum states. This article reviews the excitonic states and coordinated interplay of charge, spin, and lattice. We discuss the recent experimental and theoretical discoveries of excitonic phenomena, as well as correlated states involving condensation and cooperative emission. Additionally, our exploration extends to the structural properties of MHPs that facilitate the emergence of robust quantum states, even at room temperatures. Finally, an overview of the remaining challenges and potential applications of MHPs in quantum optics, coherent light sources, electrically driven amplified spontaneous emission, and superfluorescent lasing is provided.

Graphical abstract

Abstract Image

金属卤化物过氧化物中激子的新集体量子现象
具有独特电子和光学特性的金属卤化物过氧化物(MHPs)已成为在光伏、光电和光子设备领域具有广泛应用前景的材料。激子和集合量子态错综复杂地定义了 MHPs 的独特性质和巨大潜力。本文回顾了激子态以及电荷、自旋和晶格的协调相互作用。我们讨论了激子现象的最新实验和理论发现,以及涉及凝聚和协同发射的相关态。此外,我们还探讨了 MHP 的结构特性,这些特性有助于即使在室温下也能产生稳健的量子态。最后,我们概述了 MHPs 在量子光学、相干光源、电驱动放大自发辐射和超荧光激光方面的其余挑战和潜在应用。
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来源期刊
Mrs Bulletin
Mrs Bulletin 工程技术-材料科学:综合
CiteScore
7.40
自引率
2.00%
发文量
193
审稿时长
4-8 weeks
期刊介绍: MRS Bulletin is one of the most widely recognized and highly respected publications in advanced materials research. Each month, the Bulletin provides a comprehensive overview of a specific materials theme, along with industry and policy developments, and MRS and materials-community news and events. Written by leading experts, the overview articles are useful references for specialists, but are also presented at a level understandable to a broad scientific audience.
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