Nuclear-excited source of coherent and incoherent radiation with direct nuclear pumping

IF 1.6 3区 工程技术 Q3 CHEMISTRY, INORGANIC & NUCLEAR
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Abstract

Uranium fission fragments, as well as the products of 3He(n,p)3H and 10B(n,α)7Li nuclear reactions were utilized in the nuclear reactor for gas ionization and excitation. However, the 6Li(n,α)3H nuclear reaction was less examined. The use of lithium-6 as a surface source of excitation of the gas medium, due to the long path length of tritium nuclei in the gas, allows to excite large volumes of gas as opposed to using 235U or 10B.

While investigating the luminescence of noble gases in the core of the IVG.1M research reactor, we noted an appearance of alkali metal lines and a sharp increase in the intensity of these lines at temperatures above 570 K. It was determined that the population of levels of lithium atoms has practically no effect on the population of the 2p-levels of atoms of noble gases. The selectivity of p- and s-levels deactivation by lithium atoms implies the possibility of creating inversion of population at 2p-1s transitions of noble gas atoms. Successful experiments to study the luminescence of gases upon excitation by 6Li(n,α)3H nuclear reaction products allow us to proceed to experiments to achieve the laser action threshold and study the lasing characteristics of gas mixtures at the IGR pulsed nuclear reactor with thermal neutron flux density up to 7∙1016 n/cm2s. For this purpose, an experimental device designs were proposed to perform experiments on the IGR reactor. A step-by-step procedure of fabrication of a nuclear-excited source for excitation of gas mixtures is provided. The results of reactor experiments aimed at determining the spectral and temporal characteristics of optical radiation during excitation of gas mixtures by 6Li(n,α)3H nuclear reaction products are presented.

具有直接核抽运功能的相干和非相干辐射核激源
核反应堆利用铀裂变碎片、3He(n,p)3H 和 10B(n,α)7Li 核反应产物进行气体电离和激发。但对 6Li(n,α)3H 核反应的研究较少。与使用 235U 或 10B 相比,使用锂-6 作为气体介质的表面激发源,由于氚核在气体中的路径长度较长,可以激发大量气体。在研究 IVG.1 M 研究反应器核心中惰性气体的发光情况时,我们注意到碱金属线的出现以及这些线在 570 K 以上温度时强度的急剧增加。锂原子对 p 级和 s 级失活的选择性意味着,在惰性气体原子的 2p-1s 转变中可能会出现原子群反转。研究气体在 6Li(n,α)3H 核反应产物激发下发光的成功实验,使我们能够在热中子通量密度高达 7∙1016 n/cm2s 的 IGR 脉冲核反应堆上进行实验,以达到激光作用阈值,并研究气体混合物的发光特性。为此,提出了在 IGR 反应堆上进行实验的实验装置设计。提供了用于激发气体混合物的核激发源的逐步制造过程。介绍了旨在确定 6Li(n,α)3H 核反应产物激发气体混合物期间光辐射的光谱和时间特征的反应堆实验结果。
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来源期刊
Applied Radiation and Isotopes
Applied Radiation and Isotopes 工程技术-核科学技术
CiteScore
3.00
自引率
12.50%
发文量
406
审稿时长
13.5 months
期刊介绍: Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.
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