B.S. Hu , Z.H. Sun , G. Hagen , G.R. Jansen , T. Papenbrock
{"title":"Ab initio computations from 78Ni towards 70Ca along neutron number N = 50","authors":"B.S. Hu , Z.H. Sun , G. Hagen , G.R. Jansen , T. Papenbrock","doi":"10.1016/j.physletb.2024.139010","DOIUrl":null,"url":null,"abstract":"<div><p>We present coupled-cluster computations of nuclei with neutron number <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> “south” of <sup>78</sup>Ni using nucleon-nucleon and three-nucleon forces from chiral effective field theory. We find an erosion of the magic number <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> toward <sup>70</sup>Ca manifesting itself by an onset of deformation and increased complexity in the ground states. For <sup>78</sup>Ni, we predict a low-lying rotational band consistent with recent data, which up until now has been a challenge for ab initio nuclear models. Ground states are deformed in <sup>76</sup>Fe, <sup>74</sup>Cr, and <sup>72</sup>Ti, although the spherical states are too close in energy to unambiguously identify the shape of the ground state within the uncertainty estimates. In <sup>70</sup>Ca, the potential energy landscape from quadrupole-constrained Hartree-Fock computations flattens, and the deformation becomes less rigid. We also compute the low-lying spectra and <span><math><mi>B</mi><mo>(</mo><mi>E</mi><mn>2</mn><mo>)</mo></math></span> values for these neutron-rich <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> nuclei.</p></div>","PeriodicalId":4,"journal":{"name":"ACS Applied Energy Materials","volume":null,"pages":null},"PeriodicalIF":5.4000,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0370269324005689/pdfft?md5=1fd0998cb302fbbe296f8a5b4c580252&pid=1-s2.0-S0370269324005689-main.pdf","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Energy Materials","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0370269324005689","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
We present coupled-cluster computations of nuclei with neutron number “south” of 78Ni using nucleon-nucleon and three-nucleon forces from chiral effective field theory. We find an erosion of the magic number toward 70Ca manifesting itself by an onset of deformation and increased complexity in the ground states. For 78Ni, we predict a low-lying rotational band consistent with recent data, which up until now has been a challenge for ab initio nuclear models. Ground states are deformed in 76Fe, 74Cr, and 72Ti, although the spherical states are too close in energy to unambiguously identify the shape of the ground state within the uncertainty estimates. In 70Ca, the potential energy landscape from quadrupole-constrained Hartree-Fock computations flattens, and the deformation becomes less rigid. We also compute the low-lying spectra and values for these neutron-rich nuclei.
期刊介绍:
ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.