Metal-organic frameworks based solid-state electrolytes for lithium metal batteries: Modifications and future prospects

Next Energy Pub Date : 2024-09-11 DOI:10.1016/j.nxener.2024.100191

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Abstract

Metal-organic frameworks (MOFs) represent a cutting-edge category of porous crystalline organic-inorganic hybrids that have attracted significant interest in the realm of energy storage and conversion. MOFs offer several advantages, including ordered channels, high specific surface area, precisely controllable structures, high functionality, and desirable physicochemical characteristics, which position them as promising candidates for solid-state electrolytes (SSEs). This review systematically explores recent efforts in the development of MOF-based SSEs for solid-state lithium metal batteries. We categorize these advancements into three key systems based on the functionalities of MOFs: (1) incorporation of guest molecules into MOFs, (2) modification of MOFs, and (3) MOFs-based composite in SSEs. We discuss the advantages and potential challenges associated with MOFs in these applications, and propose key design strategies and emerging trends. This review aims to offer innovative insights and practical guidance for the development of MOF-based electrolytes.

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基于金属有机框架的锂金属电池固态电解质：改性与未来展望

金属有机框架（MOFs）是多孔结晶有机无机杂化物的一个前沿类别，在能量存储和转换领域引起了极大的兴趣。MOFs 具有多种优势，包括有序通道、高比表面积、结构精确可控、高功能性和理想的物理化学特性，这些都使其成为固态电解质 (SSE) 的理想候选材料。本综述系统地探讨了最近在开发基于 MOF 的固态锂金属电池 SSE 方面所做的努力。我们根据 MOFs 的功能将这些进展分为三个关键系统：(1) 将客体分子加入 MOFs；(2) MOFs 的改性；(3) 基于 MOFs 的 SSE 复合材料。我们讨论了 MOFs 在这些应用中的优势和潜在挑战，并提出了关键设计策略和新兴趋势。本综述旨在为开发基于 MOF 的电解质提供创新见解和实用指导。

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Next Energy

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