Dynamic flexoelectric instabilities in nematic liquid crystals

Abstract

Electrohydrodynamic phenomena in liquid crystals constitute an old but still very active research area. The reason is that these phenomena play the key role in various applications of liquid crystals and due to the general interest of the physical community in out-of-equilibrium systems. Nematic liquid crystals (NLCs) are ideally representative for such investigations. Our article aims to study theoretically the linear NLCs dynamics. We include into consideration orientation elastic energy, hydrodynamic motion, external alternating electric field, electric conductivity, and flexoelectric polarization. We analyze the linear stability of the NLC film, determining dynamics of perturbations with respect to the homogeneous initial state of the NLC. For the purpose we compute eigenvalues of the evolution matrix for a period of the external alternating electric field. These eigenvalues determine the amplification factors for the modes during the period. The instability occurs when the principal eigenvalue of the evolution matrix becomes unity by its absolute value. The condition determines the threshold (critical field) for the instability of the uniform state. It turns out that one might expect various types of the instability, only partially known and investigated in the literature. Particularly, we find that the flexoelectric instability may lead to two-dimensionally space-modulated patterns exhibiting time oscillations. This type of the structures was somehow overlooked in the previous works. We formulate conditions needed for the scenario to be realized. We hope that the results of our work will open the door to a broad range of further studies. Of especial importance would be a comprehensive understanding of the role of various material parameters and nonlinear effects which is a key step for the rational design of NLCs exhibiting the predicted in this publication multidimensional oscillating in time patterns.