Proton beam based production of positron emitters by exploiting the 27Al(p,x)22Na reaction

Abstract

Positron annihilation experiments on an laboratory scale depend on the supply and the availability of ${\beta }^{+}$ emitters. Here we present the production of positron sources based on the ²⁷Al(p,x)²²Na reaction by irradiation of Al with a 68 MeV proton beam. We simulated the energy loss, range and radial scattering of the protons in Al in order to design a simple target consisting of a stack of Al discs. Our approach allows (i) the direct use of the Al discs as positron emitters that inherently avoids wet chemical processes as usually applied in commercial production of carrier-free ²²Na, (ii) the production of multiple positron sources at once, and (iii) the simple measurement of the depth and lateral distribution of ²²Na. We precisely determined the cross section of the ²⁷Al(p,x)²²Na reaction which was found to differ from literature values particularly for proton energies between 27 and 40 MeV. The activity of all nuclides produced (apart from ²²Na) was shown to be negligible 15 days after irradiation. The production of radionuclides such as ⁴⁸Sc, ⁵⁴Mn and ⁵⁶Co can be prevented by using Al of a higher purity. The concept presented here can easily be adapted for the production of stronger ²²Na sources by increasing the proton current or/and the irradiation time.